Abstract
To identify and quantify the sediment sources in the South Sea of Korea, a marginal sea of the northwestern Pacific, we analyzed a comprehensive aluminum–magnesium dataset comprising 121 surface sediment samples and two sediment cores. The findings demonstrate pronounced spatial variation in sediment sources, with Korean river sediments dominating in embayment bays and Chinese river sediments prevailing in the shelf area. In the coastal zone, Korean river sediments account for over 60–70%, but their proportion decreased to 10–20% in the shelf zone. This reveals that most of the sediments from Korean rivers are mainly confined to the coastal embayments, with limited transport to the shelf area. Notably, the central South Sea mud (CSSM) deposits are primarily govern by the sediment influx from Chinese rivers (CR), rather than the Seomjin River discharge. The prevalence of CR-sourced sediments in the shelf region is closely linked to the Tsushima Warm Current and Cheju Warm Current, transporting sediments from the East China Sea shelf northwards and the southwestern Korean coastal zone eastwards, respectively. This driving mechanism for the widespread deposition of CR sediments is further supported by an abrupt shift from KR to CR dominance in sediment sources around 8 kyr BP, coinciding with the establishment of the modern current systems in the northwestern Pacific marginal seas. Our study provides a new perspective on the source-to-sink pathways, particularly of Chinese river sediments, in the formation of the Korean coastal mud deposits.
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1 Introduction
Deciphering sediment provenance and distribution pathways in marginal seas that encompass extensive river systems is pivotal for comprehending historical variations in paleoceanography and paleoclimate (Milliman and Meade 1983; Allen 2017; Zhao et al. 2018). In view of this, the sediment source-to-sink pathways and the associated deposition processes in the Yellow Sea and the northern East China Sea (YECS), which are the epitome of epicontinental shelves in the northwestern Pacific marginal sea, have been rigorously conducted over recent decades (e.g., Park and Khim 1992; Cho et al. 1999, 2015; Yang et al. 2003; Yang and Youn 2007; Lim et al. 2020 and references therein). Remarkably, this body of research has zeroed in on the distinct mud patch deposits found in the YECS shelf (Fig. 1a), yielding valuable insights into the evolution of oceanic circulation systems and the complex interactions between land and ocean, often associated with climate shifts (Li et al. 2014; Hu et al. 2014a, b; Wang et al. 2014; Lim et al. 2015a and references therein). Moreover, these source-to-sink studies have uncovered the evolving influences of the Huanghe and Changjiang rivers in the formation of shelf mud deposits (Hu et al. 2014b; Dou et al. 2015; Lim et al. 2015a; Koo and Cho 2020), as well as the intricate mechanisms behind their formation, including the current systems of gyres and/or upwellings (Hu 1984; Shi et al. 2003; Bian et al. 2013; Wang et al. 2014).
Another intriguing revelation from source-to-sink investigations is the identification of sediments originated from Chinese rivers (CR) within the Korean coastal deposits. An earlier study on probing sediment sources highlighted a discrepancy between the total sediment budget and sediment contributions from Korean rivers (KR) within Korean coastal zones, hinting at the presence of supplementary sediment influx (Park et al. 2000; Lim et al. 2007). Subsequent studies employing clay mineral and elemental proxies reinforced the notion that these additional sediments primarily stemmed from the Changjiang and/or the Huanghe (e.g., Cho et al. 2015; Um et al. 2015; Kwak et al. 2016; Lim et al. 2013, 2020). In particular, these Korean coastal mud deposits displayed elevated contents of smectite and some elements (e.g., iron, magnesium, and heavy rare earth elements) which are characteristic of CR sediments. This finding implies a considerable inflow of fine-grained sediments originating from Chinese rivers to the Korean coastal zones, particularly since around 6–8 kyr BP (Lim et al. 2020).
Despite the breadth of sediment source-to-sink research, dispersal patterns and quantities of sediments emanating from Chinese rivers remain contested topics, particularly in regard to the South Sea shelf of Korea, characterized by extensive mud deposits (Bae et al. 2014; Um et al. 2017; Kim et al. 2019; Lee, et al. 2019, 2023). The prevailing view has been that fine-grained sediments in the South Sea, especially within the inner shelf region, predominantly originate from Korean rivers, with the Seomjin and Nakdong Rivers being the major contributors (Fig. 1b). Nevertheless, the spatial extent of sediment dispersion from Korean rivers has not been definitively ascertained. Recently, Um et al. (2017) posited that sediments from Chinese rivers might have partially contributed to the formation of the thick mud deposit on the inner shelf of the central South Sea, known as the Central South Sea Mud (CSSM). However, this ‘multi origin’ hypothesis regarding the CSSM has yet to achieve consensus due to the scarcity of compelling evidence. Furthermore, the precise extent of CR source contributions to the South Sea shelf region, including the CSSM, remains to be clarified.
Various clay mineralogical and elemental proxies for discerning sediment sources in YECS mud deposits have been developed (e.g., Yang et al. 2003 and references therein; Xu et al. 2009; Lim et al. 2014, 2015a, b; Dou et al. 2015; Koo et al. 2018; Jung et al. 2021). Among these, alkaline earth elements, such as magnesium (Mg) and iron (Fe), have been widely acknowledged as reliable elemental markers for distinguishing different sources of fine-grained sediments in the YECS, as they exhibit distinct linear regression trends between groups of KR and CR sediments in correlation with aluminum (Al) (Lim et al. 2006a, 2013; Koo et al. 2018). Recently, an innovated approach for source quantification based on the advanced Al–Mg regression model was proposed, and this has been instrumental in achieving quantitative estimations of sediment source contributions (Lim et al. 2020). This methodology holds promise for more decisive sediment source discrimination in the South Sea of Korea, and for deepening our comprehension of sediment source-to-sink dynamics in the northwestern marginal seas.
In this study, our objectives are to distinguish and quantify the contributions of sediment sources from Chinese rivers (Changjiang and Huanghe) in the South Sea of Korea through the analysis elemental compositions of fine-grained sediments (with a mean grain size > 4ϕ), with particular emphasis on Al and Mg data. The relative contributions of each source for the samples were calculated using the Al–Mg regression method as outlined by Lim et al. (2006a, 2020). We collected a total of 79 surface sediment samples from the coastal and shelf regions of the South Sea of Korea (Fig. 1b). To gain a more encompassing portrayal of the spatial–temporal variations in sediment sources across the entire South Sea region, we also compiled and assessed data from prior studies. This approach enables us to capture and analyze nuanced information on sediment sources across the South Sea, thereby providing a comprehensive perspective on sediment dynamics within the region.
2 Regional Setting
The South Sea of Korea, situated at the northern extremity of the East China Sea, is bordered to the north by the numerous postglacial embayments and small islands, constituting a quintessential ria-type coast (Fig. 1a). The bathymetry is generally parallel to the coastline and extend to the E–W direction on the western part of the sea but turns to the NE–SW direction on the eastern part. The sediments are mostly composed of the modern fine sediments on the inner shelf and send deposits on the outer shelf (Chough et al. 2000). Notably, the central area of the sea is distinguished by presence of the thick Holocene shelf mud deposits (i.e., CSSM) up to 20–30 m, which have accumulated since the last glacial maximum concurrent with the rise in sea levels (Park et al. 1996). The Seomjin and the Nakdong Rivers, the largest rivers flowing into the South Sea, contribute approximately 0.8 × 106 ton year−1 and 4.6–10 × 106 ton year−1, respectively (Lim et al. 2007 and references therein), to the coastal and inner shelf zones of the sea. The hydrodynamic conditions in the sea are primarily influenced by the northeastward Tsushima Warm Current (TWC), a branch of Kuroshio Current, and the coastal current in conjunction with Cheju Warm Current (CWC) which courses eastward along the southern coastline. Given these geographic and oceanographic characteristics, a reconstruction of the spatial and temporal variations in sediment sources in the South Sea may provide valuable insights into the dispersion limits of KR and/or CR sediments, as well as the evolution of TWC system over time.
3 Materials and Methods
Grain size analysis for surface sediments was performed using a standard dry-sieving technique for sand-sized fractions (> 63 μm), and a pipette method for mud fractions (silt- and clay-sized fractions; < 63 μm) after the removal of calcium carbonate and organic compounds. Textural parameters were calculated using the graphic method based on the weight percentages of each phi fraction (Ingram 1971). For the elemental contents (i.e., Al and Mg) of bulk sediments, each powdered sediment sample was fused with lithium meta-borate (LiBO2) flux and the molten beads were subsequently poured into a volume of dilute nitric acid and agitated until dissolved. The resultant solutions were analyzed using a Thermo iCAP 6500 radial inductively coupled plasma optical emission spectrometer. Standard reference material (MAG-1) was analyzed alongside a batch of sediment samples and the relative deviations between measured and certified values were found to be less than 5%. Analytical results, including previously reported data, are presented in Table 1.
In this study, the quantification of sediment sources is based on the Al–Mg regression model as proposed by Lim et al. (2006a, 2020). Briefly, the relative contributions of each sample were computed by calculating perpendicular distances between the position of a sediment sample on a scatter plot and each of the Al–Mg linear regression lines corresponding to KR and CR sediment groups (Fig. 2a). Specifically, the coordinates of the intersection point of the two regression lines representing KR and CR sediments were shifted to serve as the origin (0, 0), as the lines were not parallel (for further details, see Lim et al. 2006a); concurrently, the Al and Mg contents of all sediment samples from the study area were adjusted in accordance with the transformed origin. This correction essentially normalizes the bulk contents of the elements, accounting for variations in grain size, thereby refining sediment geochemistry.
In this study, a new Al–Mg linear regression line for the Korean river source was generated based on the combined data of the western Korean rivers (Lim et al. 2020) and the Seomjin River (Fig. 2a). This comprehensive dataset allowed more robust analysis and accurate estimation of source contributions for the sediments in the South Sea of Korea. The Al and Mg data of the Seomjin River are from fine surface sediments (Nam 2016) and short push-core sediments from the lower reaches of the river (Lim, personal communication). To ensure robust data collection and interpretation, furthermore, data from previous studies, including 42 surface sediment samples (Cho 1994) and two sediment core (Lee et al. 2019), were integrated with the newly acquired data (refer to Fig. 1b for sample sites).
4 Results and Discussion
In this study, we examined grain sizes and Al and Mg contents of 121 surface sediments and two sediment cores, incorporating previous data, to deepen our understanding of sediment sources, with a particular emphasis on their quantitative contributions in the entire South Sea shelf. The surface sediments mainly comprise fine-grained muds, with mean grain sizes ranging from 4.32 to 9.70 ϕ (average: 7.53 ± 1.33 ϕ) (Fig. 3a). The content of mud (silt + clay) exceeds 80% (range: 33 to 100%) in most of the sediments, whereas the sand content is generally below 10% (Fig. 3b). The Al2O3 and MgO contents in surface and core sediments range from 8.59 to 23.26% (average: 14.69 ± 2.33%) and 1.27 to 3.22% (average: 2.35 ± 0.40), respectively (Fig. 3c, d). Notably, their spatial variations are aligned with the mean grain size distribution.
Mg has been established as a definitive tracer for identifying sediment provenance in the YECS. The Al–Mg correlation plot distinctly reveals different linear regression lines for the KR and CR sediments (Fig. 2a), signifying a marked difference in Mg content between the two groups, despite similarities in grain size. This divergence in Mg content is ascribed to the contrasting source rocks in each river basin. Sediments from Korean rivers are predominantly characterized by higher contents of quartz and potassium feldspar, whereas sediments from Chinese rivers contain a greater proportion of mafic rocks, including an abundance of ferromagnesian minerals and plagioclase feldspars (Lim et al. 2014, 2015b). Interestingly, in the Al–Mg discrimination plot, surface sediments from the study area are distributed between the KR and CR sources and exhibit distinct linear regression trends that deviate from those of the KR and CR sediments (Fig. 2b), suggesting that the surface sediments comprise a combination of both sources. This observation enables estimation of the relative contributions from each source by measuring the perpendicular distances between the position of a sediment sample and each of the KR and CR linear regression lines (Fig. 2a).
Our quantitative source estimates across the South Sea region unambiguously demonstrate a spatial demarcation between contributions from the KR and CR sources (Fig. 4). Importantly, the spatial variation in sediment source is gradual from the coastal dominated by the Korean river source to the shelf zones overwhelmed by the Chinese river source, which is parallel to overall bathymetric contour in the study. The findings show that most of the sediments in the study area represent a mix of these sources, corroborating earlier findings (Um et al. 2017; Lee et al. 2019). In particular, the coastal zones are predominantly influenced by KRs sources, which account for over 60% of the total contribution. This trend is especially prominent in bays directly influenced by rivers and streams, such as the Seomjin and Nakdong Rivers (Fig. 4). Conversely, the shelf area is primarily composed of sediments sourced from Chinese rivers, making up 60–90% of the total volume (Fig. 4). This significant contribution from Chinese rivers to the South Sea shelf can be attributed to the considerable influx of the TWC, which carries energy (e.g., heat and moisture) and materials (e.g., nutrients and particulates) from the East China Sea to the South Sea of Korea and the YECS. This suggests an extensive offshore supply originating from the northern East China Sea shelf, where large quantities of fine-grained sediments, either from the Huanghe or Changjiang accumulated (Lim et al. 2007; Youn and Kim 2011; Hu et al. 2014b; Dou et al. 2015). Consequently, the high deposition of CR sediments in Korea’s shelf regions results from the transport of reworked sediments from the East China Sea shelf along the TWC pathway, particularly during the winter season.
Meanwhile, the transport of CR sediments from the shelf regions to coastal embayment zones appears to be influenced by strong tidal currents and their asymmetry in magnitude between flood and ebb in the embayment coastal areas. Specifically, hydrodynamic observation data from the Yeosu Sound, connected to Gwangyang Bay, indicated higher concentrations of suspended sediments in the near-bottom water and a pattern of tidal asymmetry with stronger flood currents (Kim and Kang 1991). This observation implies that the amount of suspended sediments entering Gwangyang Bay through the Yeosu Sound surpasses the quantity transported out of the bay, highlighting that fine offshore and shelf sediments can be effectively transported to coastal embayment regions. Hence, the combination of stronger flood currents and higher concentration of suspended sediments near the bottom plays a crucial role in the deposition of CR sediments in the coastal embayments of the South Sea.
Another possible mechanism for the high contribution of CR sediments in the South Sea of Korea is the influence of the CWC, which branches off from the TWC and forms a robust eastward flow, circulating clockwise around Jeju Island. This current transports a substantial quantity of suspended particulate matter, estimated at approximately 23 × 106 ton year−1 (Chung et al. 2000), into the South Sea. This is comparable to the total sediment loads of all Korean rivers, which range from ~ 11 to 39 × 106 ton year−1, Lim et al. 2007). Recent studies have proposed that sediments reworked from the Southeastern Yellow Sea Mud (SEYSM) (Heuksan Mud Belg, HMB) deposits along the southwestern Korean coastal zone are carried into the South Sea by the CWC (Um et al. 2017; Lee et al. 2019). The SEYSM deposits, representative of offshore mud deposition in Korea, comprise multiple sediment sources (Kwak et al. 2016; Lim et al. 2020 and reference therein), including CR sediments, which contribute about 50% of the total deposition (Park et al. 2017; Lim et al. 2020). Hence, the spatial variations in sediment sources within the South Sea shelf are strongly influenced by the TWC and/or CWC, which transport sediments originating from the Changjiang- and/or Hunanghe from the northern East China Sea shelf and/or the southern SEYSM deposits.
Despite potential uncertainties in our quantitative estimates, it is evident that sediment derived from CR sources plays a crucial role in forming the shelf mud deposits in the South Sea of Korea, constituting more than 60% of the total sediment budget. This finding provides a compelling explanation for the discrepancy previously noted between the volumes of KRs sediment inputs and the accumulation budget of muddy deposits in Korean coastal zones. For instance, the Nakdong and the Seomjin Rivers discharge approximately 0.8 × 106 ton year−1 and 4.6–10 × 106 ton year−1 of particulate matter, respectively, into the South Sea (Lim et al. 2007 and references therein). However, the sediment budgets of these Korean rivers are deemed insufficient to explain the formation of the thick mud deposits in the coastal and inner shelf regions of the South Sea (Lim et al. 2007; Bae 2015; Lee et al. 2023). Furthermore, our findings suggest that most sediments from Korean rivers are retained within coastal embayments along the shoreline, with only minimal amount being transported into the shelf region (Fig. 4).
An additional significant aspect of this study is the temporal variation in sediment sources observed in two well-dated sediment cores from the CSSM deposits developed on the inner shelf of the South Sea (Fig. 5). Similar to the surface sediments, all core sediment samples exhibit a scattered distribution between the KR and CR sediments (Fig. 2b), indicative of a mixture of both sources. The proportion of CR sediments in the cores varied between 20 and 70% over time, suggesting substantial temporal changes in sediment source-to-sink dynamics. Of particular note is the abrupt shift from KRs sediment dominance to CR sediment dominance around 8 kyr BP (Fig. 5). Prior to approximately 8–10 kyr BP, the CSSM deposits were primarily composed of KR sediments, accounting for over ~ 75% of total sediment budget. However, during the late-to-middle Holocene after ~ 8 kyr BP, there was a relatively high contribution of CR sediments (approximately 50–70%). This sudden and marked shift in the dominant sediment source is closely linked the evolution of the ocean current system in response to the incursion of the TWC, coupled with rising sea level.
The prevailing sea-level low-stand before the Holocene led to the seaward extension of the coastline and the emergence of the exposed shelf in the South Sea of Korea. In the study area, the paleo-shoreline was located approximately 60 km southeast of its present position, and rivers such as the Seomjin River stretched southward, resulting in the incision of the continental shelf (Park et al. 2000; Bae et al. 2018). Notably, sediments from the paleo-Seomjin River accumulated within the widely developed incised valleys on the modern shelf of the central South Sea (Bae et al. 2014, 2018; Lee et al. 2017). During this period, the Chinese rivers (i.e., the Huanghe and Changjiang) flowed into the edge of the East China Sea shelf near the northern Okinawa Trough (Li et al. 2015; Xu et al. 2017). Besides, it is probable that the TWC was either absent or extremely weak in the epi-continental shelf regions of the northwestern Pacific marginal seas, including the South Sea, during this time (Diekmann et al. 2008; Lim et al. 2015a; Xu et al. 2014). Consequently, the contributions from paleo-Chinese Rivers to the South Sea of Korea were minimal or non-existent. Thus, the central South Sea shelf was mainly filled with the Seomjin River-sourced sediments during the sea-level low-stand before approximately 8 kyr BP, leading to a high proportion of KRs sources in sediment cores.
With the rise in sea level during the Holocene, the coastline and the mouths of Korean rivers likely receded gradually, causing most of the KR sediments to be trapped within the present estuaries and coastal embayments, as evidenced by the high proportion of KR sources depicted in Fig. 4. Concurrently, the shelf environmental system was governed by oceanic currents, especially the TWC, which facilitated the extensive northward transport of CR-sourced sediments from Chinese rivers across the East China Sea shelf. In addition, the Changjiang Diluted Water plume (Fig. 1a) contributed to the northeastward movement of some Changjiang sediments, particularly during intense monsoon seasons. Therefore, the sudden increase in the CR source contribution since around 8 kyr BP could be attributed to the intrusion of the TWC into the study area. Moreover, this temporal shift in sediment sources coincides with the notion that the postglacial sea-level rise was nearly completed by around 8 kyr BP, at which point the modern oceanic circulation patterns were established. Studies examining the development of the TWC, particularly in the Korean Strait and the Hupo Basin of the southeastern Korean shelf, support our interpretation that the TWC likely stabilized at this time and flowed into the East/Japan Sea through this strait (Lim et al. 2006b; Khim et al. 2021).
This historical progression of sedimentation and the ocean current system is evident in sediment core (YSDP 102 and 103, refer to Fig. 1b for core sites) from the southern part of the SEYSM deposit along the southwestern coasts of Korea. As indicated in Fig. 5, in these cores, the contribution of CR sediments also increased significantly since around 8 kyr BP, which demonstrate a tentative correlation between the sediment source variation and the onset of Yellow Sea Warm Current (YSWC) inflow into the Yellow Sea (Lim et al. 2020). In the Yellow Sea at this time, the dominant sediment source remarkably changed to the Changjiang, while the supplies from Huanghe decreased (Lim et al. 2015a). This noticeable change is also associated with the formation of the modern surface water circulation system with the dominance of the YSWC and the Yellow Sea coastal current (YSCC) mainly controlled riverine supply to the CYSM, while the importance of estuary shift, tidal stress, sea-level fluctuation, and monsoon climate change was significantly weakened. With respect to its relevance to historical sedimentary deposits of the YECS sediments over the last approximately 14 kyr BP (Fig. 5), our fingerprint-inferred provenance changes depict a distinct sedimentation trend over the course of the Holocene, marked by a substantial increase in the CR contribution since around 8 kyr BP. Nonetheless, determining the precise onset timing of ocean circulation systems and their final formation coupled with sea level rise in the northern Pacific marginal seas (i.e., the Yellow Sea, South Sea of Korea, and East/Japan Sea) necessitates further investigation through the comprehensive correlation of well-dated sediment cores.
As shown in the core 16PCT-GC03 (Fig. 5), besides, the sedimentation rate in the shelf region significantly increased from ~ 0.37 m/ka during the middle Holocene (~ 8.5 to ~ 3.12 ka) to ~ 1.12 m/ka since ~ 3 ka. This increase is also evident in another sediment core (SSDP103) from the CSSM deposit: in this sediment core, the sedimentation rate is low at ~ 2.47 m/ka in the middle Holocene, but increased more than five times (~ 10.20 m/ka) during the late Holocene (data from Kong et al. 2013). The results suggest that sediments originating from the East China Sea and/or the southwestern Korean coastal zone were deposited at much higher sedimentation rates as sea level rise slowed or stabilized during the late Holocene. The relatively high sediment deposition during the late Holocene may be linked to strengthened YSWC and CWC since ~ 4 ka (Kong et al. 2006; Li et al. 2009), leading to enhanced sediment supply from the northern East China Sea (e.g., ECSDM) and the SEYSM; however, temporal changes in the sedimentation rates and sediment sources in the sediment cores from additional locations will be necessary for better defining the long-term depositional mechanism in the shelf zone of the South Sea.
5 Conclusions
In this study, we analyzed a comprehensive dataset that encompasses the Al and Mg contents from surface sediment samples and two sediment cores, integrating previously reported data. Objective of this study was to scrutinize the spatial and temporal variations in the sources of these sediments throughout the entire South Sea region, inclusive of the coastal and shelf zones. To quantitatively estimate the sediment sources, we used the Al–Mg regression model, which unearthed notable spatial variations in the contributions from Korean and Chinese rivers. In the coastal zone of the South Sea, KR sediments constitute over 60–70% of the total; however, this proportion drops to 10–20% in the shelf zone. This finding signifies that most of the sediments from Korean rivers are confined within the coastal embayments along the shoreline, with only a scant amount extending into the shelf region. In contrast, the shelf regions of the South Sea are predominantly blanketed by fine-grained sediments that originate from Chinese rivers, accounting for over 70% of the total sediment budget. This underscores the significant influence of CR sediments on the formation of muddy deposits in the central South Sea, lending credence to the multi-source concept for the CSSM. Besides, our results delineate a distinct sedimentation trend over the course of the Holocene period, characterized by a substantial increase in the contribution of CR sediments commencing around 8 kyr BP. This depositional history of shelf mud deposits is intimately connected to the evolution of the TWC inflow. By quantifying and elucidating the sediment sources throughout the South Sea, this research enhances our understanding of the sediment routing system and depositional evolution of mud depositions in the marginal sea with large rivers, such as the Huanhge and the Changjiang.
Data availability
The original contributions presented in the study are given in the article.
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Acknowledgements
This work was supported by National Research Foundation of Korea (grant no. NRF-2022R1A2C1006208) and Korea Institute of Marine Science & Technology (KIMST) funded by the Ministry of Oceans and Fisheries (RS-2023-00256330, Development of risk managing technology tackling ocean and fisheries crisis around Korean Peninsula by Kuroshio Current). We thank the Library of Marine Sample (LIMS), Korea Institute of Ocean Science and Technology (KIOST) for supplying the samples.
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Lim, D., Cho, YG., Jeong, D. et al. A Comprehensive Investigation of Coastal and Shelf Sediment Sources in the South Sea of Korea: A Marginal Sea of the Northwestern Pacific. Ocean Sci. J. 58, 28 (2023). https://doi.org/10.1007/s12601-023-00121-2
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DOI: https://doi.org/10.1007/s12601-023-00121-2