Abstract
Predicting the dynamics of quantum systems far from equilibrium represents one of the most challenging problems in theoretical many-body physics1,2. While the evolution of a many-body system is in general intractable in all its details, relevant observables can become insensitive to microscopic system parameters and initial conditions. This is the basis of the phenomenon of universality. Far from equilibrium, universality is identified through the scaling of the spatio-temporal evolution of the system, captured by universal exponents and functions. Theoretically, this has been studied in examples as different as the reheating process in inflationary Universe cosmology3,4, the dynamics of nuclear collision experiments described by quantum chromodynamics5,6, and the post-quench dynamics in dilute quantum gases in non-relativistic quantum field theory7,8,9,10,11. However, an experimental demonstration of such scaling evolution in space and time in a quantum many-body system has been lacking. Here we observe the emergence of universal dynamics by evaluating spatially resolved spin correlations in a quasi-one-dimensional spinor Bose–Einstein condensate12,13,14,15,16. For long evolution times we extract the scaling properties from the spatial correlations of the spin excitations. From this we find the dynamics to be governed by an emergent conserved quantity and the transport of spin excitations towards low momentum scales. Our results establish an important class of non-stationary systems whose dynamics is encoded in time-independent scaling exponents and functions, signalling the existence of non-thermal fixed points10,17,18. We confirm that the non-thermal scaling phenomenon involves no fine-tuning of parameters, by preparing different initial conditions and observing the same scaling behaviour. Our analogue quantum simulation approach provides the basis with which to reveal the underlying mechanisms and characteristics of non-thermal universality classes. One may use this universality to learn, from experiments with ultracold gases, about fundamental aspects of dynamics studied in cosmology and quantum chromodynamics.
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Main
Isolated quantum many-body systems offer particularly clean settings for studying fundamental properties of the underlying unitary time evolution19. For systems initialized far from equilibrium, different scenarios have been identified, including the occurrence of many-body oscillations20 and revivals21, the manifestation of many-body localization22, and quasi-stationary behaviour in a prethermalized stage of the evolution23.
Here we observe a new scenario associated with the notion of non-thermal fixed points. This is illustrated schematically in Fig. 1a: starting from a class of far-from-equilibrium initial conditions, the system develops a universal scaling behaviour in time and space. This is a consequence of the effective loss of details about initial conditions and system parameters long before a quasi-stationary or equilibrium situation may be reached. The transient scaling behaviour is found to be governed by the transport of an emergent collective conserved quantity towards low momentum scales.
For our experimental study we employ an elongated Bose–Einstein condensate of about 70,000 87Rb atoms. We use the F = 1 hyperfine manifold with its three magnetic sublevels mF = 0, ±1 as a spin-1 system with ferromagnetic interactions24. Initially, all atoms are prepared in the mF = 0 sublevel, forming a spinor condensate with zero spin length. The dynamics is initiated by instantaneously changing the energy splitting of the F = 1 magnetic sublevels by means of microwave dressing (see Methods). Consequently, spin excitations develop in the Fx–Fy plane12 as sketched in Fig. 1b. Our experimental setup allows the extraction of the spin distribution in terms of the spin component \({\hat{F}}_{x}\left(y\right)=\left[{\hat{\psi }}_{0}^{\dagger }\left(y\right)\left({\hat{\psi }}_{+1}^{}\left(y\right)+{\hat{\psi }}_{-1}^{}\left(y\right)\right){\rm{+h}}{\rm{.c}}{\rm{.}}\right]/\sqrt{2}\) where \({\hat{\psi }}_{m}^{\dagger }\left(y\right)\) is the creation operator of an atom in the magnetic sublevel m at position y and h.c. denotes the Hermitian conjugate. At a given time t this is achieved by a spin rotation from the Fx–Fy plane to the Fz-direction and subsequently detecting the atomic density difference Fz(y) = n+1(y)− n−1(y) (see Methods for details). Representative absorption images are shown in Fig. 1c together with the extracted spin profiles (green lines). The histograms in Fig. 1c show the probability distribution of Fx for all positions y and experimental realizations for the corresponding evolution time (see Extended Data Fig. 1 for all evolution times). Results are presented for characteristic stages associated with the initial condition (1), the nonequilibrium instability regime (2), the universal scaling regime (3) and the departure from the non-thermal fixed point (4), as also indicated in Fig. 1a.
We find that during the time evolution the angular orientation θ of the transverse spin (see Fig. 1b) becomes the relevant dynamical degree of freedom. For short evolution times unstable longitudinal spin modes grow exponentially25, well described by Bogoliubov theory, but nonlinear evolution quickly takes over (after about 100 ms). This leads to a double-peaked structure of the histograms (see Fig. 1c) indicating that the spin has a mean length and a random orientation in the Fx–Fy plane. On the basis of this observation we extract the mean spin length \(\langle |{F}_{\perp }(t)|\rangle \), where F⊥ = Fx + iFy, and its fluctuations using a fit. Building on that knowledge, we extract the local angle from the profiles as \(\theta (y,t)={\rm{a}}{\rm{r}}{\rm{c}}{\rm{s}}{\rm{i}}{\rm{n}}({F}_{x}(y,t)/\langle |{F}_{\perp }(t)|\rangle )\) (see Methods for details).
The time evolution of the fluctuations of the spin orientation is described in terms of correlation functions of the scalar field θ(y,t). The fluctuations are analysed by evaluating the two-point correlation function C(y,y ′;t) = 〈θ(y,t)θ(y ′,t)〉. To distinguish the role of different length scales we consider a momentum-resolved picture of the dynamics. Hence we evaluate the structure factor, which is the Fourier transform of C(y,y ′;t) with respect to the relative coordinate \(\bar{y}={y}^{^{\prime} }-y\), averaged over y:
In general, the structure factor fθ is a function of momentum k which evolves in time t in a way determined by the system parameters and initial conditions. In Fig. 2a, we plot fθ(k,t) as a function of k on a double-logarithmic scale for times between 4 s and 9 s. A characteristic shift of the structure factor towards smaller momenta as well as an increase of the low-momentum amplitude with time is observed.
In fact, instead of separately depending on k and t we find that in this regime the datasets collapse to a single curve if the rescaled distribution t−αfθ is plotted as a function of the single variable tβk. This implies that the data satisfy the scaling form
with universal scaling exponents α, β and scaling function fs. Figure 2b shows this collapse, where the same data points as in Fig. 2a are plotted with times normalized to the reference time tref = 4.5 s. The ability to reduce the full nonequilibrium time evolution of the correlation function in the scaling regime to a time-independent, so-called fixed-point distribution fs(k) and associated scaling exponents is a striking manifestation of universality.
We find the amplitude scaling exponent to be α = 0.33 ± 0.08 and the momentum scaling exponent to be β = 0.54 ± 0.06. The errors correspond to one standard deviation obtained from a resampling technique (see Methods). However, the actual uncertainty for α is expected to be larger since the rescaling analysis is much less constraining on α than on β. We find that fθ(k,t) develops a plateau at the lowest momenta and an approximate power-law fall-off above a characteristic length scale in the scaling regime. To parameterize the universal scaling function, we fitted the rescaled data with a function of the form26: fs(k) ∝1/[1 + (k/ks)ζ] and find ζ ≈ 2.6, with ks ≈ 1/133 µm−1 for our system. The value of ζ becomes constant after about 4 s (see Fig. 3a). Analysing fθ(k = 0, t) as shown in Fig. 3b reveals that the occupation of k = 0, which cannot be seen on the logarithmic scale employed in Fig. 2, builds up in the scaling regime. This growth is consistent with the power law proportional to tα with α obtained from the rescaling analysis, as indicated by the solid line. After 9 s the system departs from the scaling behaviour.
The nature of the observed scaling phenomenon is explained by the emergence of an approximately conserved quantity and its transport. In terms of our dynamical degree of freedom θ(y,t) we identify ∫dk〈|θ(k,t)|2〉 ≡ ∫dk fθ(k,t) as the conserved quantity. In fact, Fig. 3c shows that the sum over all modes k for different evolution times—after a fast initial rise due to the instability—settles around a constant within the scaling regime (see also Extended Data Fig. 2). According to the scaling (2), ∫dk fθ(k,t) = tα−β∫dk fs(k) ≈ const. corresponds to α ≈ β so that in our case only one independent dynamical scaling exponent remains. A distinct feature is the transport of the conserved quantity directed towards the infrared, corresponding to a positive sign of β. Theoretically it is expected to find the scaling only for momenta smaller than some scale10 (in our case about 0.04 µm−1; see Extended Data Fig. 3). The transport towards the infrared is in contrast to the turbulent transport into the ultraviolet observed in direct cascades27.
These experimental findings of scaling behaviour, implying universality, allow comparison with predictions in a variety of models in the non-thermal universality class, which is defined by the scaling function fs and α = dβ for given spatial dimension d. N interacting Bose gases with equal intra- and interspecies Gross–Pitaevskii couplings are described by an O(N) symmetric model. This is closely related to O(N) symmetric scalar models28, such as the relativistic Higgs sector of the Standard Model with N = 4 for d = 3. For these types of models, both Gross–Pitaevskii and relativistic, a universal value of β ≈ 0.5 has been predicted and found to be insensitive to the spatial dimension10 for d ≥ 2. This describes the self-similar transport of excitations of the relative phases between the components to lower wavenumbers. The scaling function fs is known to depend on dimensionality29 and has not yet been theoretically estimated for d = 1. Our setup is, to our knowledge, the first realization of an effective N = 3 model for the transport of conserved quantities associated with non-thermal fixed points in a quasi-one-dimensional situation. Finding scaling behaviour in one dimension was not expected and sheds new light on the concept of universality classes far from equilibrium.
We emphasize that the non-thermal scaling phenomenon studied here involves no fine-tuning of parameters. This is in contrast to equilibrium critical phenomena, which require a careful adjustment of system variables, such as the temperature, to a critical value30. To illustrate this insensitivity we employ the high level of control of the atomic spin system and prepare three qualitatively different initial conditions (for details see Methods). The corresponding absorption images of single realizations are shown in Fig. 4a along with the Fourier transform of the spatial correlation function of Fx(y).
We find universal dynamics for all initial conditions with comparable inferred scaling exponents (see inset of Fig. 4b). We rescale the data with the same exponents obtained from the mean of all four measurements and take into account overall scaling factors and reference momentum scales. This procedure leads to a collapse of all data, manifesting the robustness of non-thermal fixed point scaling.
The level of control demonstrated here and the accessible observables on our platform open the door to the discovery of further non-thermal universality classes. This represents a crucial step towards a comprehensive understanding of out-of-equilibrium dynamics with potential impact in various fields of science.
(We note that similar phenomena have recently been observed by the Schmiedmayer group31 in Vienna in a single-component Bose gas, where a scaling exponent β ≈ 0.1 was extracted.)
Methods
Microscopic parameters
The dynamics of the spinor Bose gas is described by the Hamiltonian
where \({\hat{n}}_{m}={\hat{\psi }}_{m}^{\dagger }{\hat{\psi }}_{m}\), with \({\hat{\psi }}_{m}^{\dagger }\) the bosonic field creation operator of the magnetic substate m ∈ {0,±1}, and : : denotes normal ordering. \({\hat{H}}_{0}\) contains the spin-independent kinetic energy and trapping potential. The spin operators are given by \({\hat{F}}_{x}=\left[{\hat{\psi }}_{0}^{\dagger }\left({\hat{\psi }}_{+1}^{}+{\hat{\psi }}_{-1}^{}\right){\rm{+h}}{\rm{.c}}{\rm{.}}\right]/\sqrt{2}\) and \({\hat{F}}_{y}=[i{\hat{\psi }}_{0}^{\dagger }({\hat{\psi }}_{+1}^{}-{\hat{\psi }}_{-1}^{})+{\rm{h}}.{\rm{c}}.]/\sqrt{2}\) and \({\hat{F}}_{z}={\hat{n}}_{+1}-{\hat{n}}_{-1}\). The parameter p describes the linear Zeeman shift in a magnetic field. For the hyperfine spin F = 1 of 87Rb the spin interaction is ferromagnetic, that is, c1 < 0.
For the experimental control parameter q > 2n|c1|, with n being the total density, the mean-field ground state is the polar state, which corresponds to all atoms occupying the mF = 0 state. In the range 0 < q < 2n|c1| a spin with non-vanishing length in the x–y plane is energetically favoured (easy-plane ferromagnet)32. This is the parameter regime employed in the experiment.
Experimental system
We prepare a Bose–Einstein condensate of about 70,000 atoms in the state (F,mF) = (1, 0) in an optical dipole trap of 1,030 nm light with trapping frequencies ωǁ ≈ 2π × 2.2 Hz and ω⊥ ≈ 2π × 250 Hz.
The control parameter q is given by q = qB − qMW, where qB ≈ 2π × 56 Hz is the second-order Zeeman splitting in a magnetic field of B ≈ 0.884 G and qMW = Ω2/4δ is the energy shift due to the microwave dressing. For dressing33 we use a power-stabilized microwave generator with resonant Rabi frequency Ω ≈ 2π × 5.3 kHz and δ ≈ 2π × 137 kHz blue detuned with respect to the (1, 0) ↔ (2, 0) transition. For the spin dynamics we adjust Ω and δ so that q ≈ n|c1| (with nc1 ≈ −2π × 2 Hz). To monitor the long-term stability of q we do a reference measurement every 4 h (corresponding to about 250 experimental realizations). For this we observe spin dynamics for a fixed evolution time of 4 s as a function of the control parameter q (changing the detuning δ). Analysing the integrated side mode population we infer that the drifts of q are well below 0.5 Hz.
Preparation of different initial conditions
We prepare three initial conditions (see Fig. 4) that differ from the polar state. For initial condition 1 the control parameter is first set to q ≈ n|c1|+1 Hz. After 500 ms of spin dynamics at this value we quench to the final value q ≈ n|c1|. For the preparation of initial condition 2 we apply a resonant π/5 radio-frequency pulse to populate the (1, ±1) states. After a hold time of 100 ms at a magnetic field gradient of around 0.2 µG µm−1 in the longitudinal trap direction we apply a second π/5 radio-frequency pulse. The combination of q and an inhomogeneous p during the hold time leads to a spatially modulated transversal spin on a length scale of λ ≈ 80 µm. For initial condition 3 we populate homogeneously the (1, ±1) states with a short radio-frequency pulse such that (n+1 + n−1)/n ≈ 0.1.
Spin read-out
The spin dynamics is initiated by quenching the control parameter. After a fixed evolution time t we apply a short magnetic field gradient pulse (Stern–Gerlach) in the z-direction and switch off the waveguide potential. Following a short time of flight (about 1 ms) we perform high-intensity absorption imaging with a resonant light pulse of duration 15 µs. The resolution of the imaging system is about 1.2 µm, corresponding to three pixels on the charge-coupled-device camera34; we accordingly bin the spin profiles by three pixels. As our Stern–Gerlach analysis is oriented in the z-direction, for the read-out of the spin in the x–y plane we apply, before the magnetic field gradient, a radio-frequency pulse resonant with the transitions (1, 0) ↔ (1, ±1).
The radio-frequency pulse can be modelled as a spin rotation described by the Hamiltonian \({\hat{H}}_{{\rm{r}}{\rm{f}}}={\Omega }_{{\rm{r}}{\rm{f}}}{\hat{F}}_{y}\) with resonant Rabi frequency Ωrf ≈ 2π × 17.5 kHz. Applying a π/2-pulse of duration 14.3 µs, the observable \({\hat{F}}_{x}\) is mapped to the measurable density difference n+1 − n−1.
Inferring the spin orientation
The double-peaked spin distributions in the scaling regime (see Extended Data Fig. 1) resemble a distribution of a transversal spin with random orientation. To extract the corresponding ensemble average length \(\left\langle \left|{F}_{\perp }\right|\right\rangle \) of the transversal spin and its fluctuation σ we fit a probability density of the form \(p({F}_{x})\propto 1/\sqrt{1-{({F}_{x}/\langle |{F}_{\perp }|\rangle )}^{2}}\) convolved with a Gaussian distribution with root-mean-square σ. Under the assumption of a homogeneous spin length the spatial profile of the angular orientation is given by \(\theta (y)={\rm{a}}{\rm{r}}{\rm{c}}{\rm{s}}{\rm{i}}{\rm{n}}({F}_{x}(y)/\langle |{F}_{\perp }|\rangle )\). If the maximal amplitude is larger than \(\langle |{F}_{\perp }|\rangle -\sigma \) we use the maximal amplitude of the single realization instead of \(\left\langle \left|{F}_{\perp }\right|\right\rangle \).
Extraction of scaling exponents
After rescaling the results of the discrete Fourier transform according to equation (2) we interpolate with cubic splines to obtain a common k-grid for all evolution times. We vary the scaling exponents α and β to minimize the sum of the squared relative differences of all structure factors fθ. To estimate the statistical error on the exponents we employ a jackknife resampling analysis35.
Data availability
The data presented in this paper are available from the corresponding author upon reasonable request.
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Acknowledgements
We thank D. M. Stamper-Kurn, J. Schmiedmayer, A. Piñeiro Orioli, M. Karl, J. M. Pawlowski and A. N. Mikheev for discussions. This work was supported by the Heidelberg Center for Quantum Dynamics, the European Commission FET-Proactive grant AQuS (project number 640800), the ERC Advanced Grant Horizon 2020 EntangleGen (project ID 694561) and the DFG Collaborative Research Center SFB1225 (ISOQUANT).
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The experimental concept was developed in discussion among all authors. M.P., P.K. and S.L. controlled the experimental apparatus. M.P., P.K., H.S., S.L. and M.K.O. discussed the measurement results and analysed the data. C.-M.S., J.B. and T.G. elaborated the theoretical framework. All authors contributed to the discussion of the results and the writing of the manuscript.
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Extended data figures and tables
Extended Data Fig. 1 Spin distributions for all evolution times.
a, The panels show the distributions of the transversal spin, Fx, measured at different evolution times as indicated. Initially, we find a narrow Gaussian distribution corresponding to the prepared coherent spin state. The excitations developing in the transversal spin lead to a double-peaked distribution within the interval of 2 s to 10 s. For long evolution times, t > 12 s, the distribution resembles a Gaussian, which is much broader than the initial distribution. b, The spin length and its root-mean-square fluctuation as a function of evolution time are extracted by a fit (see Methods). We find a slow decay of the spin length and nearly constant root-mean-square fluctuations in the scaling regime.
Extended Data Fig. 2 Build-up of transversal spin in momentum space.
Since the angular orientation θ cannot be extracted reliably for short evolution times, we choose to show the Fourier transform of the transversal spin for regimes 1–3 (see Fig. 1). The initial condition, all atoms prepared in mF = 0, is characterized by a flat distribution. There is a fast build-up of long-wavelength spin excitations by more than two orders of magnitude within the first second. This process is followed by a redistribution of momenta leading to the scaling form for times longer than 4 s.
Extended Data Fig. 3 Scaling of structure factor for all experimentally accessible length scales.
Same data as shown in Fig. 2. a, Unscaled data. b, Data rescaled with the scaling exponents reported in the main text. The rescaling does not apply for large momenta, k > 0.04 µm−1.
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Prüfer, M., Kunkel, P., Strobel, H. et al. Observation of universal dynamics in a spinor Bose gas far from equilibrium. Nature 563, 217–220 (2018). https://doi.org/10.1038/s41586-018-0659-0
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DOI: https://doi.org/10.1038/s41586-018-0659-0
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