Abstract
Flexible device is widely used in wearable device, biosensors, soft robotics, and foldable/rollable display, and still a lot of potential application are ahead. In this review, fabrication techniques and materials for flexible devices will be referred to. In the end, issues related with the commercialization of the flexible device will be discussed.
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Introduction
Flexible Device and its Prospect
Flexible devices are called electronic devices with high stretch ratio, which can be used in various applications. Most representative examples of commercial flexible devices are rollable-foldable displays, which were first introduced by SAMSUNG Display and LG Display [1, 2]. Other applications of the flexible devices are health and biomedical devices which can be used as wearable sensors for monitoring physiological parameters like heart rate, body temperature, and blood pressure, or monitoring health metrics such as glucose levels, hydration, and UV exposure (BioStamp Research Connect, MC10) [3,4,5,6]. Other application of the flexible device is soft robots which can adapt to their environment and are equipped with flexible electronic sensors and actuators [7,8,9,10,11].
Advancement and commercialization of flexible devices will give chances to bring new products in our life. Haptic [12,13,14,15,16] device with AR / VR display [17,18,19] is one of the possible usages of flexible device, which will be suitable interface for meta services [20,21,22,23]. Both exterior and interior part of the vehicle will be totally changed when flexible display become patchable into multi-curved surface. The interior cockpit of the vehicle will be changed into a full display panned which eliminates blind spots, as shown in Fig. 1.
Methods for Mass Production in Flexible Device
Most of the methods for fabricating flexible devices can be categorized into three: (1) Printing techniques [24,25,26,27,28,29], (2) Lithography and deposition methods [30,31,32,33,34,35], and (3) Hybrid and Roll-to-Roll process [36,37,38,39,40,41,42,43]. In the case of printing techniques, these methods are generally cost-effective and scalable, making them suitable for mass production. However, compared to lithography, printing techniques have relatively low yield rate, lower resolution, and material viscosity constraints, which can limit their applicability in certain scenarios.
Lithography and deposition techniques offer high resolution and the ability to create precise, high-quality features, often essential for specialized applications. However, they can be time-consuming, require expensive equipment, and may have limitations in terms of scalability and material compatibility.
In the case of hybrid and roll-to-roll processes, these methods are designed for high-throughput, continuous production and allow for the integration of different types of materials and components. However, they may require complex processes, have alignment challenges, and can be constrained by material compatibility and resolution limits.
Detailed methods with advantages and limitations are listed in Table 1.
Material and Structure Design in Flexible Device
Numerous materials and designs have been developed for stretchable electronics, and their scale are varied from mm to nano scale. The use of composite materials such as conductive polymers integrated into elastomers can provide both mechanical durability and electrical conductivity [44,45,46,47,48,49]. In situ polymerization methods are used to blend the materials at the molecular level, enhancing stretchability. Nanowires, nanotubes, and nanoparticles have been embedded into elastomeric substrates to provide conductivity while maintaining stretchability [50,51,52,53,54,55]. Materials like liquid metal alloys are adopted in making stretchable circuits. The intrinsic properties of these materials allow them to maintain conductivity even under strain. Incorporating self-healing polymers as a substrate can provide long-term durability [56,57,58,59,60,61,62,63,64]. Any ruptures or cracks in the material can be automatically healed, maintaining electrical conductivity, as shown in Table 2.
Instead of changing materials, implementing mechanical designs such as origami or kirigami can help in fabricating stretchable electronic devices. These designs can accommodate mechanical deformations while maintaining the functionality of the device. Incorporating microfluidic channels filled with liquid metal into elastomeric substrates can offer excellent electrical conductivity while maintaining stretchability, as shown in Table 3 [65,66,67,68,69,70,71,72,73,74].
Barrier for Commercialization of Flexible Devices.
Even if some stretchable electronics has been successively commercialized, still there are issues which hinders the advance of stretchable electronics. One of the main obstacles in the design and mass production of flexible electronics is getting vast volumes of material characteristics and device performance to be consistent and homogeneous. Also, manufacturing processes must be scalable in order to be able to adjust and optimize the efficiency of mass production. Balancing material costs with performance poses challenges in sourcing reliable and cost-effective materials in large quantities [79, 80]. The cost for stretchable conductive material is high due to the nano-materials such as Ag nanowire, CNT, Au nanoparticle, and the stacking of the device in unit area are limited due to the structure of the device itself [75,76,77,78]. The complex fabrication methods often require specialized equipment and controlled environments, adding to the cost.
Using mechanical patterns such as origami or kirigami in flexible electronics has its drawbacks. Firstly, complex folding patterns could eventually increase the concentration of mechanical stress, which could compromise the structural integrity of the device [85, 86]. Secondly, the intricacy of these designs could make mass production less efficient because they call for precise folding and assembly, which could be difficult to accomplish on a large scale [87, 88]. Furthermore, frequent folding and unfolding could cause wear and tear, which would reduce its long-term dependability. Achieving a balance between robustness and intricate designs that can be produced in large quantities is crucial in these kinds of applications [89]. Repeated stretching and relaxation cycles can lead to material fatigue, causing cracks or delamination in conductive pathways or substrates [79,80,81,82,83,84,85,86]. Uneven distribution of mechanical strain can lead to "hot spots" where failure is more likely to occur.
Poor adhesion between different material layers can result in delamination or peeling, especially under mechanical stress. Such mechanical degradation eventually causes conductivity degradation, and Joule heating problem of the device [87,88,89,90,91,92,93]. Several strategies can be used to improve Adhesion between distinct material layers in stretchable electronics and lower the possibility of delamination or peeling under mechanical stress [105,106,107]. Material surfaces can be altered by surface treatments like chemical or plasma treatments to enhance bonding [108]. Adhesion can be improved by using interfacial materials that are compatible or adhesion-promoting intermediary layers [109, 110]. Other successful tactics include designing flexible substrates with intrinsic adhesion-promoting qualities and optimizing material selection. Furthermore, investigating cutting-edge adhesive technologies—like bio-inspired adhesives or functionalized polymers—can strengthen the interlayer bonding in flexible electronic devices [111,112,113,114].
Conclusion
Stretchable electronics has been developed for more than a decade and commercialized products are now at hand. However, their cost for production is high, and development of reliable, high resolution, and energy effective devices are still becoming issues for advance of the flexible devices.
Future research in the manufacturing of flexible electronics should primarily concentrate on the development of novel materials that are more flexible, robust, and functional; self-healing technologies, biocompatible materials, and effective energy harvesting are important areas to be maximized. It will be of great importance to also address the issues of scalability and cost-effectiveness in future research works. Mass manufacturing of flexible electronics also need to give ethical standards, environmental sustainability, and human welfare top priority.
Data availability
The data used or analyzed during the preparation of this review paper are derived from published literature and publicly available databases. All references to the original sources are provided within the manuscript. No new data were generated specifically for this review.
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Acknowledgement
This work was supported by the National Research Foundation of Korea (NRF) grant funded by the Korea government (MSIT) (No. 2021R1F1A1051120).This results was supported by "Regional Innovation Strategy (RIS)" through the National Research Foundation of Korea(NRF) funded by the Ministry of Education(MOE) (2021RIS-004).
Funding
Jung-Hoon Yun has received research support from Korea government (MSIT) (No. 2021R1F1A1051120), and Ministry of Education (2021RIS-004). Oluwabukola Adebisi has no financial interest in this study.
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Yun, JH., Adebisi, O. Issues Related with Commercialization and Mass Production of Flexible Devices. Multiscale Sci. Eng. 5, 126–132 (2023). https://doi.org/10.1007/s42493-024-00099-6
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DOI: https://doi.org/10.1007/s42493-024-00099-6