We propose a new approach for catalyst development that combines different scientific disciplines: experimental design, surface science, reaction kinetics and simulations with the objective of accelerating catalyst development. In this paper we present a study of the possibilities of using small data sets in microkinetic modeling, and studies of the required precision of temperature measurement.
Article PDF
Similar content being viewed by others
Avoid common mistakes on your manuscript.
References
G.F. Froment and K.B. Bischoff, Chemical Reactor Analysis and Design (John Wiley and Sons, 1990)
D.T. Lynch G. Emig (1989) Chem. Eng. Sci. 44 IssueID6 1275 Occurrence Handle10.1016/0009-2509(89)85001-8 Occurrence Handle1:CAS:528:DyaL1MXkt1Gltb0%3D
A. Corma F. Llopis J.B. Monton S.W. Weller (1988) Chem. Eng. Sci. 43 IssueID4 785 Occurrence Handle10.1016/0009-2509(88)80073-3 Occurrence Handle1:CAS:528:DyaL1cXkt1yiu7c%3D
P. Stoltze J.K. Nørskov (1988) J. Catal. 110 1 Occurrence Handle10.1016/0021-9517(88)90291-6 Occurrence Handle1:CAS:528:DyaL1cXitFWjur0%3D
J.K. Nørskov T. Bligaard A. Logadottir S. Bahn L.B. Hansen M. Bollinger H. Bengaard B. Hammer Z. Sljivancanin M. Mavrikakis Y. Xu S. Dahl C.J.H. Jacobsen (2002) J. Catal. 209 275 Occurrence Handle10.1006/jcat.2002.3615
C.J.H. Jacobsen, Chem. Commun. (2000) 1057
J.A. Moulijn J. Perez-Ramirez R.J. Berger G. Hamminga G. Mul F. Kapteijn (2003) Catal. Today 81 457 Occurrence Handle10.1016/S0920-5861(03)00145-7 Occurrence Handle1:CAS:528:DC%2BD3sXlsVWrsLk%3D
J. Perez-Ramirez R.J. Berger G. Mul F. Kapteijn J.A. Moulijn (2000) Catal. Today 60 93 Occurrence Handle10.1016/S0920-5861(00)00321-7 Occurrence Handle1:CAS:528:DC%2BD3cXkslWlsLw%3D
P. Stoltze (2000) Progr. Surf. Sci. 65 65 Occurrence Handle10.1016/S0079-6816(00)00019-8 Occurrence Handle1:CAS:528:DC%2BD3cXmtFGju70%3D
H. Lynggaard A. Andreasen C. Stegelman P. Stoltze (2004) Progr. Surf. Sci. 77 71 Occurrence Handle10.1016/j.progsurf.2004.09.001 Occurrence Handle1:CAS:528:DC%2BD2cXpslWgsbk%3D
R.J. Barlow (1989) Statistics: A Guide to the Use of Statistical Methods in Physical Sciences John Wiley and Sons Chichester
T. Bligaard K. Honkala A. Logadottir J.K. Nørskov S. Dahl C.J.H. Jacobsen (2003) J. Phys. Chem. B 107 9325 Occurrence Handle10.1021/jp034447g Occurrence Handle1:CAS:528:DC%2BD3sXmtVCnu74%3D
Author information
Authors and Affiliations
Corresponding author
Rights and permissions
About this article
Cite this article
Hansen, A.G., van Well, W.J.M. & Stoltze, P. Microkinetic modeling as a tool in catalyst discovery. Top Catal 45, 219–222 (2007). https://doi.org/10.1007/s11244-007-0269-9
Issue Date:
DOI: https://doi.org/10.1007/s11244-007-0269-9