Abstract
The total quantity of data available on the 119Sn Mössbauer resonance is now quite considerable, but the application of this resonance has not had quite the same impact on chemistry as has that of 57Fe. In the latter isotope many of the effects observed result from the sensitivity of the 3d-orbitals to the chemical environment. However, these remain essentially non-bonding or antibonding in all but the most covalent compounds, and thus retain a degree of identity which allows full and successful use of ligand field theory. We have already seen in Chapter 9 that the results on diamagnetic covalent compounds of iron are more difficult to interpret in detail, and this is also true for most of the compounds of tin since our knowledge of the chemical binding involved is equally rudimentary. The tin atom does not carry an intrinsic spin moment in any of its compounds, and consequently magnetic hyperfine splitting is only found in rather rare circumstances. In the absence of large applied magnetic fields, therefore, this considerably limits the information obtainable.
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Greenwood, N.N., Gibb, T.C. (1971). Tin-119. In: Mössbauer Spectroscopy. Springer, Dordrecht. https://doi.org/10.1007/978-94-009-5697-1_14
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