Abstract
A zirconium-based metal organic framework (UiO-66-NH2) was prepared using a greener approach for the removal of hexavalent chromium (Cr(VI)) from solution. The characterization of UiO-66-NH2 was performed using several methods, and the influence of the solution pH, adsorbent dosage, salt, adsorption time, Cr(VI) concentration and adsorption temperature on adsorption quantity was performed in batch mode. UiO-66-NH2 can efficiently remove Cr(VI) through the synergistic effect of adsorption and reduction. At pH solution of 1.1 and solid-to-liquid ratio of 2 g·L−1, the removal rate of 100 mg·L−1 Cr(VI) increased to 95.2%. The maximum adsorption capacity of UiO-66-NH2 from Langmuir model was 252 mg·g−1. The adsorption equilibrium process can be well described by Langmuir, Koble-Corrigan and Temkin models, while the kinetic process can be predicted by pseudo-second-order and Elovich model. UiO-66-NH2 showed a good adsorption capacity in a wide range of pH (pH=1.1–10) and also had better regeneration performance after five cycles using 0.01 mol·L−1 NaOH; consequently, it can be a promising adsorbent for the removal of Cr(VI) from solution.
Article PDF
Similar content being viewed by others
Explore related subjects
Discover the latest articles, news and stories from top researchers in related subjects.Avoid common mistakes on your manuscript.
References
A. K. Deb, B. Biswas, R. Nadu and M.M. Rahman, J. Hazard. Mater., 421, 126812 (2022).
B. Valizadeh, T. N. Nguyen, S. Kampouri, D. T. Sun, M. D. Mensi, K. Stylianou, B. Smit and W. L. Queen, J. Mater. Chem. A, 8, 9629 (2020).
Q. Li, X.B. Cai, L.H. Chen, B.B. Guan, Z.L. Fan, W. Zhu and D. X. Xue, Inorg. Chem., 60, 8143 (2021).
T.C. Nguyen, X. T. Nguyen, D.M.T. Tran, Q.T. Vu, V.H. Nguyen, D. T. Nguyen, M. T. Do, T. L. Nguyen, T. N. L. Ly and H. Thai, Bioinorg. Chem. Appl., 2020, 1 (2020).
T. Kekes, G. Kolliopoulos and C. Tzia, J. Environ. Chem. Eng., 9, 105581 (2021).
J. S. Marciano, R. R. Ferreira, A. G. de Souza, R. F. S. Barbosa, A. J. de Moura Junior and D.S. Rosa, Int. J. Biol. Macromol., 181, 112 (2021).
S. X. Dong, Y.L. Wang, J.Y. Li, D.X. Zhang, Y.Q. Zhou and Y. Tong, Chem. Eng. J., 394, 124944 (2020).
M. S. Samuel, E. Selvarajan, R. Chidambaram, H. Patel and K. Brindhadevi, Chemosphere, 284, 131368 (2021).
L. L. Fang, L. Ding, W. Ren, H. Q. Hu, Y. Huang, P. H. Shao, L. M. Yang, H. Shi, Z. Ren, K. K. Han and X. B. Luo, J. Hazard. Mater., 416, 125829 (2021).
X. M. Chen, W. G. Zhang, X. L. Luo, F. Zhao, Y. X. Li, R. H. Li and Z. H. Li, Chemosphere, 185, 991 (2017).
R. Khosravi, G. Moussavi, M. T. Ghaneian, M. H. Ehrampoush, B. Barikbin, A. A. Ebrahimi and G. Sharifzadeh, J. Mol. Liq., 256, 163 (2018).
F. Bahador, R. Foroutan, H. Esmaeili and B. Ramavandi, Carbohyd. Polym., 251, 117085 (2021).
A. Hosseinkhani, B. Forouzesh Rad and M. Baghdadi, J. Environ. Manage., 274, 111153 (2020).
A. Zubair, H. N. Bhatti, M. A. Hanif and F. Shafqat, Water Air Soil Pollut., 191, 305 (2008).
A. R. Iftikhar, H. N. Bhatti, M. A. Hanif and R. Nadeem, J. Hazard. Mater., 161, 941 (2009).
M. Akram, H. N. Bhatti, M. Iqbal, S. Noreen and S. Sadaf, J. Environ. Chem. Eng., 5, 400 (2017).
S. S. Kahu, A. Shekhawat, D. Saravanan and R. M. Jugade, Carbohyd. Polym, 146, 264 (2016).
K. Y. A. Lin, Y. T. Liu and S. Y. Chen, J. Colloid Interface Sci., 461, 79 (2016).
S. S. Chen, Z. Y. Zang, S. S. Zhang, G. F. Ouyang and R. P. Han, J. Environ. Chem. Eng., 9, 104780 (2021).
L. Joseph, B. Jun, M. Jang, C. M. Park, J. C. Muñoz-Senmache, A. J. Hernández-Maldonado, A. Heyden, M. Yu and Y. Yoon, Chem. Eng. J., 369, 928 (2019).
M. Sarker, J.Y. Song and S. H. Jhung, Chem. Eng. J., 331, 124 (2018).
X. Fang, S. B. Wu, Y. H. Wu, W. Yang, Y. L. Li, J. Y. He, P. D. Hong, M. X. Nie, C. Xie, Z. J. Wu, K. S. Zhang, L. T. Kong and J. H. Liu, Appl. Surf. Sci., 518, 146226 (2020).
X. Y. Liu, K.O. Kirlikovali, Z. J. Chen, K.K. Ma, K.B. Idrees, R. Cao, X. Zhang, T. Islamoglu, Y. L. Liu and O. K. Farha, Chem. Mater., 33, 1444 (2021).
X. T. Zhang, M. Y. Liu and R. P. Han, J. Environ. Chem. Eng., 9, 106672 (2021).
M. Zahid, D. X. Zhang, X. Y. Xu, M. Pan, M.H. Ul Haq, A.T. Reda and W. G. Xu, J. Hazard. Mater., 416, 125835 (2021).
S. T. Zhuang, R. Cheng and J. L. Wang, Chem. Eng. J., 359, 354 (2019).
X. Y. Shi, X. D. Zhang, F. K. Bi, Z. H. Zheng, L. J. Sheng, J. C. Xu, Z. Wang and Y. Q. Yang, J. Mol. Liq., 316, 113812 (2020).
F. Zhao, W. X. Yang, Y. Han, X. L. Luo, W. Z. Tang, T. L. Yue and Z. H. Li, Chem. Eng. J., 407, 126744 (2021).
S. Lin, D. H. Kumar Reddy, J. K. Bediako, M. Song, W. Wei, J. Kim and Y. Yun, J. Mater. Chem. A, 5, 13557 (2017).
M. M. Zhang, Q. Sun, Y. J. Wang, W. J. Shan, Z. N. Lou and Y. Xiong, Chem. Eng. J., 421, 129748 (2021).
Z. W. Chang, Y. J. Lee and D. J. Lee, J. Environ. Manage, 247, 263 (2019).
C. Wang, C. Xiong, Y. L. He, C. Yang, X. T. Li, J. Z. Zheng and S. X. Wang, Chem. Eng. J., 415, 128923 (2021).
X. Z. Jia, B. Zhang, C. Chen, X. Fu and Q. Huang, Carbohyd. Polym., 253, 117305 (2021).
M. Q. Zheng, X. D. Zhao, K. K. Wang, Y. B. She and Z. Q. Gao, Ind. Eng. Chem. Res., 58, 23330 (2019).
V. T. Trang, L. T. Tam, N. Van Quy, V. N. Phan, H. Van Tuan, T. Q. Huy, N. X. Dinh and A. Le, J. Sci.-Adv. Mater. Dev., 5, 392 (2020).
Y. X. Lai, F. Wang, Y. M. Zhang, P. Ou, P. P. Wu, Q. L. Fang, Z. Chen and S. Li, Chem. Eng. J., 378, 122069 (2019).
F. M. Mpatani, A. A. Aryee, A. N. Kani, Q. H. Guo, E. Dovi, L. B. Qu, Z. H. Li and R. P. Han, Chemosphere, 259, 127439 (2020).
C. H. Ma, X. T. Zhang, K. Wen, R. Wang and R. P. Han, Korean J. Chem. Eng., 38, 135 (2021).
M. Y. Liu, Z. Y. Zang, S. S. Zhang, G. F. Ouyang and R. P. Han, Int. J. Biol. Macromol., 182, 1759 (2021).
H. N. Bhatti, Z. Mahmood, A. Kausar, S. M. Yakout, O. H. Shair and M. Iqbal, Int. J. Biol. Macromol., 153, 146 (2020).
M. Forghani, A. Azizi, M. J. Livani and L. A. Kafshgari, J. Solid State Chem., 291, 121636 (2020).
A. A. Aryee, F. M. Mpatani, Y. Y. Du, A. N. Kani, E. Dovi, R. P. Han, Z. H. Li and L. B. Qu, Environ. Pollut., 268, 115729 (2021).
J. L. Wang, X. Liu, M.M. Yang, H.Y. Han, S.S. Zhang, G.F. Ouyang and R. P. Han, J. Mol. Liq., 338, 116698 (2021).
E. Dovi, A. A. Aryee, A. N. Kani, F. M. Mpatani, J. J. Li, Z. H. Li, L. B. Qu and R. P. Han, J. Environ. Chem. Eng., 9, 106310 (2021).
Acknowledgements
This work was financially supported by the Henan province basis and advancing technology research project (142300410224). The authors also acknowledge Farid Mzee Mpatani for improving the scientific language of this manuscript.
Author information
Authors and Affiliations
Corresponding author
Additional information
Supporting Information
Additional information as noted in the text. This information is available via the Internet at www.springer.com/chemistry/journal/11814.
Supporting Information
Rights and permissions
About this article
Cite this article
Zhang, X., Zhang, S., Ouyang, G. et al. Removal of Cr(VI) from solution using UiO-66-NH2 prepared in a green way. Korean J. Chem. Eng. 39, 1839–1849 (2022). https://doi.org/10.1007/s11814-021-1015-x
Received:
Revised:
Accepted:
Published:
Issue Date:
DOI: https://doi.org/10.1007/s11814-021-1015-x