Abstract
The magnetic, transport and acoustic properties of materials TmXMn1−XSe (0.025 ≤ X ≤ 0.2) have been studied in magnetic fields of up to 12 kOe at temperatures of 80‒600 K. The magnetic phase transition temperatures (TN) and change in the sign of resistance at DC current in vicinity of the TN were established. The temperature and concentration ranges corresponding to the maximum magnetoresistance (− 50% for X = 0.025) and magnetoimpedance (12% for X = 0.2) have been determined. The mechanism of relaxation has been established from the impedance spectrum and the activation energy change upon temperature and concentration has been found. The difference between the dc and ac magnetoresistances has been disclosed. The concentration range with hole and electron type carriers is determined. The mobility anomalies in the vicinity of the valence transition have been established. It is shown that the current and electrical resistance in the TmXMn1−XSe compound can be manipulated by ultrasound and a magnetic field. A qualitative difference between the interaction of current and ultrasound in the magnetically ordered and paramagnetic regions is found.
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Acknowledgements
The morphology of the polycrystalline TmXMn1-XSe (0.025 ≤ X ≤ 0.2) samples was examined using equipment’s (SEM) the Krasnoyarsk Regional Center of Research equipment of Federal Research Center «Krasnoyarsk Science Center SB RAS». The authors would like to express their deepest gratitude to the researcher A.I. Galyas and leading researcher K.I. Yanushkevich from Scientific-Practical Materials Research Center NAS, Minsk for the synthesis and magnetic research of samples TmXMn1-XSe.
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This work was within the state assignment of Kirensky Institute of Physics.
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All authors contributed to the study conception and design. Material preparation, data collection and analysis were performed by O.B. Romanova, S.S. Aplesnin, M.N. Sitnikov, L.V. Udod and A.M. Zhivulko. The first draft of the manuscript was written by O.B. Romanova and all authors commented on previous versions of the manuscript. All authors read and approved the final manuscript.
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Romanova, O.B., Aplesnin, S.S., Sitnikov, M.N. et al. Magnetotransport and acoustic effects in variable valence element-substituted manganese selenides. J Mater Sci: Mater Electron 35, 1751 (2024). https://doi.org/10.1007/s10854-024-13521-4
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DOI: https://doi.org/10.1007/s10854-024-13521-4