Abstract
The use of multiple-pulse laser excitation to control molecular responses that produce the ultrafast optical Kerr effect in order to perform selective spectroscopy of the Raman-active motions of molecules in liquids is discussed. Theoretical analysis and experimental data indicate that multiple-pulse laser excitation is a powerful spectroscopic tool that allows unique information to be obtained about low-frequency molecular dynamics in a liquid.
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Original Russian Text © V.G. Nikiforov, V.S. Lobkov, V.V. Samartsev, 2018, published in Izvestiya Rossiiskoi Akademii Nauk, Seriya Fizicheskaya, 2018, Vol. 82, No. 8, pp. 1108–1112.
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Nikiforov, V.G., Lobkov, V.S. & Samartsev, V.V. Selective Spectroscopy Based on the Multiple-Pulse Excitation of the Ultrafast Optical Kerr Effect. Bull. Russ. Acad. Sci. Phys. 82, 1004–1007 (2018). https://doi.org/10.3103/S1062873818080324
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DOI: https://doi.org/10.3103/S1062873818080324