Abstract
Sudden release of combustible/flammable materials at high pressure could result in the occurrence of a jet fire in the processing industry. Understanding the jet fire phenomenon and its mechanism could assist practitioners and researchers to predict the radiant energy transfer caused by the jet fire. Due to the dynamics of jet fire occurrence, the development of a semi-empirical model to predict thermal characteristics in different scenarios might provide huge advantages to the industry and safety practitioners as it is nonexpensive and a reliable prediction. There are four semi-empirical models for jet fire thermal radiation estimation that has been developed to date, namely, solid flame model (SFM), single-point source model (PSM), multipoint source model (MPSM), and line source model (LSM). It is the aim of this paper to explore each model applicability and approach to estimate the radiant heat flux based on the governing factors associated with the models, i.e., atmospheric transmissivity, flame length, lift-off length, flame shape, radiant heat fraction, total heat release, and receiver location. It is found that the applicability of each model and the derived parameters are largely contributed by the flame scale (small, medium, and large), flame orientation, flame length, and flame shape as well as the flame distance to the target receiver. From the discussion made, it can be suggested that for both near- and far-field measurement, the weighted MPSM is a reliable model that can be used for both vertical and horizontal orientations with some modification upon the consideration of buoyancy effect. On another note, LSM is able to provide a better prediction for linear trajectory of jet flame; however, the applicability is still limited for jet flame trajectory with buoyancy effects due to fewer data available and validation in various release conditions and scenarios.
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Introduction
Fire can take many different forms. The hazards associated with fire are always in the form of radiant heat release. Fire can be remotely dangerous if the sources are not contained. There are three different forms of fire that can result from the release of gas or liquid hydrocarbon as illustrated in Fig. 1.
This study focuses on jet fire occurrence which is often associated with high momentum release, promoting air entrainment which elevates the combustion efficiency. In the event of jet fire, a gas flowing at internal pressure (Pin) influences the jet exit velocity, in which if the Pin increases, the jet exit velocity would increase until it reaches a maximum condition (velocity of sound in the gas). This condition is known as a sonic or choked flow. Most released gases reached sonic velocity if the release pressure is greater than 1.9 bar absolute. A choked condition is reached if the following criteria are fulfilled:
where Pin is the internal pressure, Pout is the pressure downstream of the jet exit, and γ is the ratio of specific heats (Palacios Rosas 2011). In addition, jet fires always show turbulent characteristics, in which the flow could be chaotic and unstable due to internal and external factors as clearly illustrated in Fig. 2.
When jet fire occurred, the hazards result in the form of radiant heat transfer and the prediction of heat emission to the surrounding can be determined by semi-empirical models. In general, semi-empirical models offer the following advantages: they are easily programmed in the computer, repetitive calculation can be done in a short time, they are economical, and they could provide a reliable prediction based on theoretical principles and experimental observation. To date, semi-empirical models are adopted by industries and safety practitioners when conducting risk assessment for the plant and process. At present, four types of semi-empirical models are available, namely, solid flame model (SFM) (Raj 2007), point source model (PSM) (Hankinson and Lowesmith 2012), multipoint source model (MPSM) (Lowesmith and Hankinson 2013), and line source model (LSM) (Zhou and Jiang 2016). The models were developed based on factors including the jet flame shape, flame length, lift-off length, release flow rate, stagnant pressure, atmospheric transmissivity, release diameter, fuel reactivity, net heat release, and measurement distance. Since radiation heat transfer is the main subject during jet fire occurrence, the understanding on the physical and mechanism of jet fire and how each semi-empirical correlation relates with theories, fundamental equations, and assumptions will be our focal discussion in this paper. The governing parameters, physics, and dynamics of jet fires are reviewed for their applicability, and the present gaps between experiments as well as the common features on all models are discussed.
Semi-empirical Model of Jet Fire
The fundamental basis of radiant heat transfer estimation in a semi-empirical model is the size, shape, and relative orientation between two surfaces and their absorptivities and emissivities (Geankoplis 2003). Theoretically, the total emissive power E of radiation energy to a given surface for a black body is a relation of emissivity ε, Stefan–Boltzmann constant σ, and temperature T
To understand the basic concept of energy flow from a hotter surface to a colder surface with intervention of media such as air, view factor V has been used to explain the phenomena. It can be defined as the energy exchange between two infinite parallel black plane and gray planes to a more complicated geometrical configuration as can be seen in Fig. 3.
Theoretically, view factor can be expressed as
The basic equation involving the heat transfer between two infinite black planes is given in Eq. (4):
where QR is the radiant heat transfer, while V and E are the view factor and emissivity, respectively. With the presence of carbon dioxide and water vapor in air that act as absorbing media, thus, the transmissivity term τ shall be included in Eq. (4) that yield further equation that is adopted in the SFM:
SFM is considered a well established model since the model is the most common method used by the industry for the consequence analysis. The applicability and suitability of each model—SFM, PSM, MPSM, and LSM—are varied, depending on the process and geometrical factors. SFM and PSM are widely used models to estimate the radiant heat of fire. The shortcomings in terms of the field of observation factor for SFM and PSM models have been addressed in MPSM and LSM models and the explanation will be explored in the next section. It should be noted that all models developed are based on certain conditions that fit the models’ best and on 1D basis. The governing equations of the said models are presented in Table 1.
Where QR is the radiant heat transfer, V is the view factor, E is the emissivity per flame area (kW m−2), τ is the transmissivity, η is the fraction of heat radiated, QT is the total heat release, S is the measurement distance normal to the receiver surface area, E′ is the emissivity per flame length (kW m−1), and φ is the angle of measurement view normal to the receiver surface area. The said parameters of all models were obtained from experimental observation and theoretical assumptions. As such, emissivity E can be estimated by knowing the dimensions of the flame or via the value of η. The total heat flux QT is based on mass flow rate of released fuel m (kg s−1) and net calorific value of the fuel H (kJ kg−1), while radiant heat fraction η is based on radiant heat released QR over total heat release QT, while distance S and φ are based on the respective sensor location. Based on the aforementioned introduction, this paper attempts to discuss the parameters reported from experimental observations which are
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i.
Field of observation.
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Geometrical features of flame that include flame shape, flame length, lift-off length, and width.
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Radiant heat fraction η is based on radiant heat released QR over total heat release QT.
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iv.
Atmospheric conditions.
General Applicability of Models in Near-Field and Far-Field Observation
A key aspect of a semi-empirical model for radiant heat estimation is the location of the receiver. Thus, to have a high accuracy of prediction, the field of observation is an important factor. In general, SFM is used for radiant heat prediction in near-field observation, while PSM is used in far-field observation in which the flame shape is not critical (Lowesmith and Hankinson 2012). Even though PSM can be used for both vertical and horizontal configurations of jet flame (Zhou et al. 2016), the applicability is limited to far field only (Hankinson and Lowesmith 2012; Lowesmith et al. 2007; Lowesmith and Hankinson 2012; Jujuly et al. 2015; Zhang et al. 2015) due to the fact that the model does not consider the flame shape in the radiant heat measurement (Hankinson and Lowesmith 2012). Not considering the effect of smoke, wind velocity, and direction is another major limitation of this model (Jujuly et al. 2015), leading to weak prediction on near-field radiation and convective flux. Figure 4 is the schematic diagram of PSM with two types of measurement distance to the receiver, S and R.
The gap experienced in the PSM model is addressed in MPSM. In MPSM, instead of assuming that radiant heat is emanated from one-point source, several points are taken, assuming that heat is radiated along the jet flame centerline. MPSM is a well-accepted model that is able to replicate data on both near- and far-field observations. Originally, there were three types of MPSM, namely, linear, curvilinear, and modified curvilinear. These models were fully described elsewhere (Crocker and Napier 1988). A simple MPSM is another type of MPSM. A model adopted by Hankinson and Lowesmith (2012), which is the weighted MPSM, has demonstrated good prediction on radiation heat released from vertical orientation on large-scale jet fire in the near field. For far-field radiation estimation, the model gives a reliable prediction within ± 20% tolerance compared to PSM (Hankinson and Lowesmith 2012). Besides, the model shows a good agreement for the near-field region when the measurement is taken at a distance halfway along the flame length (Zhou and Jiang 2016). Figure 5 shows the schematic diagram of how the estimation is made using the MPSM model.
In order to determine the weight at each point, wj, which is one of the parameters in MPSM, a correlation is proposed by Hankinson and Lowesmith (2012) as shown in Eq. (10):
Hankinson and Lowesmith (2012) have established the applicability of weighted MPSM in the far-field radial distance up to 5 L. As can be seen in Fig. 6, as radial distance increases, and so is the normalized incident radiation. The value becomes close to unity at 2.5 L and 5 L of radial distance, indicating that the prediction of weighted MPSM is approximated to PSM when using distance, R. According to Zhou et al. (2016), PSM gives a good consistency on radiation measurement when the distance is more than twice the flame diameter in the horizontal direction.
In the case of near-field observation, it can be seen in Fig. 7a that the weighted MPSM and LSM show good consistency with the experimental data of Baillie et al. (1998) for small-scale jet fire in horizontal orientation, while for SFM using cylindrical shape as an assumption, the estimation gives the right trend for a radial distance more than 0.2 m. The underestimation of SFM in a radial distance less than 0.2 m may be due to incorrect flame shape assumption and this can be attributed to the buoyancy effects on the horizontal jet flame. In contrast, the simple MPSM overestimates the prediction. A possible explanation for the contrast might be due to the weight of the distributed point along the jet flame centerline is assumed to be same in simple MPSM, while for weighted MPSM, the weight at each point is calculated as described by Eq. (10).
Flame Geometrical Features
Flame geometrical features are often used in radiant heat release prediction and possible impingement to the surrounding. Thus, it is very important to know the jet flame geometrical features. Flame geometrical features are usually determined through visual observation or photograph using visible flame emission (Becker and Liang 1978), infrared flame emission (Laboureur et al. 2016), or ultraviolet flame emission (Schefer et al. 2006). Geometrical features that best represent the jet flames should be carefully evaluated including the flame shape, length, width, and lift-off length to model the heat flux (Laboureur et al. 2016). The intensity of radiant heat release to the surrounding is directly proportional to release conditions that include release mass flow rate, release pressure, jet exit velocity, momentum, release diameter, and type of fuels. In SFM and LSM, the flame shape and its corresponding dimension are a function of the release condition factors, while in PSM and MPSM, the flame length and lift-off length are correlated with the release condition factors. It can be said that the factors are intercorrelated with each other, where at higher stagnant pressure and larger exit diameter, it will result in higher jet exit velocity, mass flow rate, and momentum (Palacios Rosas 2011). Eventually, it will produce longer jet flame, thus higher emissivity value and overall heat transfer to the surrounding. Flame geometrical features that will be discussed include the following:
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Flame shape
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Flame length
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Lift-off length
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Flame width
Flame Shape
Assumption on jet fire flame shape is a common approach when using SFM and LSM predictions. The important aspect of the radiant heat transfer is the dimension and shape of the flame (Rajendram et al. 2015). Several shapes have been proposed in terms of release orientation. For vertical orientation, cylinder (Gómez-Mares et al. 2010; Hankinson and Lowesmith 2012; McCaffrey 1989), cone, back-to-back cone, back-to-back weighted ellipsoidal (Hankinson and Lowesmith 2012), and tilted cylinder (Rajendram et al. 2015) are among the flame shapes to describe the jet flame as given in Figs. 8 and 9. Cylinder, frustum of cone, ellipse, and kite flame shapes are favorable to the horizontal orientation as illustrated in Fig. 10 (Zhou et al. 2016; Zhang et al. 2015).
In general, the cylinder is often used as the flame shape for both horizontal and vertical orientations (Palacios and Casal 2011; Zhang et al. 2015; Palacios et al. 2012). For subsonic exit velocity, several flame shapes are proposed, i.e., elliptical and cylindrical. To the authors’ knowledge, limited research was conducted to determine the flame shape at sonic exit velocity. Palacios Rosas (2011) in her study proposed that the radiating cylinder shape should be taken to represent the jet flame shape on vertical release into the quiescent environment at subsonic and sonic exit velocities. The radiating cylinder uses the radiant flame length LIR as the flame length and the equivalent diameter Deq is described as the flame width obtained from the 2D area (AIR) of the jet fire surface determined by an algorithm developed in MATLAB through infrared image.
In a study done by Laboureur et al. (2016), they recommended that rectangle and kite shapes best represented the horizontal flame shape for radiation measurement. An earlier study by Sonju and Hustad (1984) on turbulent propane and methane jet flame found that emissivity E increases linearly with respect to flame length and has a good agreement with the work carried out by Kozanoglu et al. (2011) on convection heat transfer. It is commonly assumed that the E value is constant over the entire flame surface. However, the assumption of an ideal flame shape may not truly represent the real flame area, and thus, the true value of emissive power E might deviate from the real value. Furthermore, the assumption made could give an error in estimating the thermal radiation intensity in the case of near-field smoke-producing hydrocarbon fires. Although the interpretation of flame shape is varied among studies when the SFM is applied, the applicability is still valid and widely used in many industrial calculations. The application of SFM is not only restricted to jet fire but to another type of fires such as a pool fire.
Zhou and Jiang (2016) proposed the modification for E based on flame length instead of flame area due to inconsistent result on thermal radiation intensity, known as emissive power per line length (EPPLL). The suggested flame shape for vertical and horizontal orientations can be seen in Figs. 9 and 10, respectively. In this context, radiant heat is assumed to be emanated from the centerline inside the jet flame volume. Thus, the resulted data is the EPPLL (kW m−1) as compared to per flame area (kW m−2) as described in the SFM, and the deviation can be reduced as much closer to the true emissivity value when using LSM for radiant heat estimation.
Based on a study conducted by Zhou and Jiang (2016), the most suitable shape to represent the small-scale vertical jet fire is back-to-back cone shape, while for bigger vertical jet release flame with a length at approximately 10 m, a combined shape of a cylinder on the upper side and of a cone on the lower site was found to be most suitable. They also found that the kite shape flame was the best fit for radiant heat estimation for medium-scale horizontal jet fire. In addition, lift-off length must be considered once using LSM for thermal radiation calculation particularly in near-field observation.
As can be seen in Fig. 11, the inclusion of lift-off holds considerable effects on the radiant heat release.
However, all assumptions made are only applicable to the perfectly horizontal-oriented jet flame. In reality, the flame shape tends to deform on horizontal jet fire due to buoyancy effects (Ekoto et al. (2014), and this condition gives underpredicted value of the fraction of heat radiated by 40% or more. The increasing optical path length between the sensor and the flame centerline is in the buoyancy-dominated region, and this condition causing the radiant heat release was not fully captured. The flame shape deformation will certainly affect the flame length correlation, and this will be discussed further in the next section. It can be summarized that flame shape is one of the important features in SFM and LSM radiant heat prediction. It gives a direct effect on the emissivity value per area (kW m−2) when using SFM and on the emissivity value per line length (kW m−1) when LSM is applied.
Flame Length
Flame length (L) is defined as the distance between the nozzle exit to the farthest flame tip and usually controlled by the mixing process of air and fuel release (Gopalaswami et al. 2016). It is one of the important geometrical features of jet flame. The flame length estimation method has evolved over time where there is no definitive method on the number of images taken or time interval. In earlier predictions of flame length, there are two common methods used: (i) models based on stoichiometric and momentum considerations and (ii) correlations based on fuel or momentum flow that takes into account the effect of buoyancy, generally of an empirical nature (Bagster and Schubacht 1996).
As technology advances, from using manual method of visual observation, to processing using software, the number of images used to estimate flame length always varies: 30 images (Røkke et al. 1994), 90 images (Sugawa and Sakai 1996), and 30–50 images or within 10 s time interval (Lowesmith and Hankinson 2013). Flame length is used to indicate the emissive power, EPPLL in LSM, and to locate the source emitter in PSM and MPSM. In PSM and MPSM, the location of a point source in which the radiant heat is emanating lies within the axis of the flame length. It is assumed that the point should be at the center for PSM and evenly distributed along the flame axis for MPSM. There are two types of MPSM that are commonly employed: simple MPSM where the weight of source points within the flame axis is similar throughout the line and weighted MPSM in which the weight can be predicted using Eq. (10) which lies within the central line axis. Hankinson and Lowesmith (2012) observed that the weighted MPSM was capable of deriving near-field and far-field radiation as compared to PSM, in which the prediction is only satisfactory for far field only.
In order to obtain the jet flame length, there are several guidelines in which the flame length is varied according to numerous factors such as fuel velocity, leak size, mass flow rate, material release density, stagnation pressure, and net heat released. An earlier study to predict flame length suggested that flame length is independent to velocity increment or may vary slightly with velocity (Hawthorne et al. 1949). However, later findings have found that flame length was a function of mass flow rate (Wertenbach 1971; Schefer et al. 2004; Palacios et al. 2009; Mogi and Horiguchi 2009; Kalghatgi 2010).
Palacios and Casal (2011) found in their study that flame length is based on heat released by combustion, stagnation pressure, outlet orifice diameter for subsonic jet flow, and fictitious diameter of the sonic jet flow. In addition, different characterizations of flame length have been proposed based on the dimensionless number of Froude (Gopalaswami et al. 2016), Richardson (Becker and Liang 1978; Kalghatgi 2010), and Reynolds (Palacios and Casal 2011). A summary of experimental works and suggested correlations for flame length as a function of mass flow rate, Reynolds number, and Froude number is presented in Table 2.
As can be seen in Fig. 12, the correlation developed by Zhou et al. (2016) can fit the horizontal jet release data of experiments (Smith et al. 2005; Zhang et al. 2015; Gopalaswami et al. 2016; Tao et al. 2016), while the correlation by Suris et al. (1978) shows a higher coefficient, indicating that the correlation for vertical jet fire may not be applicable to horizontal jet fire. Furthermore, the applicability of flame length correlations based on Froude number is more suitable for subsonic jet release (Palacios Rosas 2011). Later findings by Schefer et al. (2006) gave an opposite observation, as they verified that the correlation is also valid for the underexpanded or sonic jet release. Another correlation was proposed as a function of jet exit diameter in the momentum-dominated regime as
where L, d, fs, ρs, and ρ∞ are the visible flame length, the jet exit diameter, the mass fraction of fuel at the stoichiometric condition, the gas density at the jet exit, and the ambient gas density, respectively. From their study, it can be deducted that the higher diameter of the nozzle exit results in higher flame length. Work done by Molina et al. (2007) gave a similar observation for flame length where the value is proportional to total jet mass flow rate and jet exit diameter.
Another correlation was proposed based on orifice’s Reynolds number based on a claim made by Palacios et al. (2009) that the value can be used for both subsonic and sonic regimes as shown in Table 2. A study by Mogi and Horiguchi (2009) suggested the correlation of the flame length as a function of stagnation pressure on their work of horizontal hydrogen jet diffusion flame at nozzle in the range of 0.1 to 4 mm from a storage pressure range of 0.01 to 40 MPa. The proposed correlation is as follows:
where L, d, and P0 are the flame length, nozzle diameter, and stagnation pressure, respectively. The correlation proposed is somewhat overestimated for flame length prediction, as reported by Studer et al. (2009) for horizontal pure hydrogen and hydrogen/methane jet release from the orifice diameter of 4, 7, and 10 mm. The proposed correlation obtained in their study is
Besides, the flame height is higher at lower atmospheric pressure as concluded by Hu et al. (2013a) when the work was carried out in a reduced atmosphere at two different altitudes—50 m (100 kPa) and 3650 m (64 kPa). For flame length, the prediction is based on heat release rate. A study for buoyancy-controlled liquefied petroleum gas (LPG) turbulent jet diffusion flame from the inclined nozzle (0°, 30°, 45°, 60°, and 90°) (Tao et al. 2016) resulted in the following expression:
where L, d, Qs*, and c2 are the flame length, nozzle diameter, dimensionless heat release rate, and constant parameter, respectively. From their study, the rate of air entrainment is proportionally inversed to the angle increment, in which lesser heat releases to the ambient when the nozzle is fully inclined to 90° (Tao et al. 2016). Thus, it implies that a higher inclination angle leads to shorter flame length, at a fixed nozzle diameter.
The previous correlation in Table 2 and Eqs. (12)–(14) was developed based on the assumption that the trajectory of the jet flame is linear; however, in real cases, the flame shape deformation would cause underprediction of radiant heat release. Ekoto et al. (2014) performed two large-scale flame experiments, using hydrogen as fuel source released from the circular nozzle with a diameter of 20.9 and 52.5 mm. The suggested method to optimize the heat source emitter in flame centerline trajectories is by employing a new developed 1D flame integral model where the mass, momentum, and mixture fraction were integrated over the flame cross-sectional area and differentiated along the flame centerline as clearly illustrated in Fig. 13.
In the case where the flame resulted is at a lower flow rate or small scale, the projection distance (Lp) is defined as the horizontal distance from the nozzle exit to the farthest point of the flame as shown in Fig. 14.
A general correlation developed is applicable for jet release from nonaxisymmetric and axisymmetric rectangular nozzles of different aspect ratios (AR = Ln/Wn) that vary from 1–1 to 71–1 where Ln is the nozzle length and Wn is the nozzle width. In this study, propane was used as fuel (Zhang et al. 2017).
where Π is the nondimensional variable defined as:
While most of the correlation developed is valid for hydrocarbon jet flame and not particularly effective for low luminosity gases such as hydrogen and syngas mixture, Miller (2017) developed a method to determine the flame length in both horizontal and vertical orientations. The method to determine overall centerline flame length is similar to Ekoto et al. (2014), where both the momentum and buoyancy region are taken into account. The flame length in the momentum region is designated as Lm, flame length in the buoyancy region is designated as Lb, and flame length with zero wind is designated as L0. The schematic diagram of jet release which accounts for buoyancy effects can be seen in Fig. 15.
The equation used for vertical jet flame is adopted from Chamberlain (1987):
The equation used for horizontal jet flame is
The overall flame length L in both orientations is
Due to the aforementioned finding of underprediction of radiant heat release due to buoyancy effects, it is therefore suggested that the buoyancy effects should be taken into consideration on the imperfect trajectory of horizontal jet fire in order to obtain a good estimation of flame length.
Lift-Off Length
Lift-off length (Lf) is another significant characteristic of jet flame as it affects the overall flame length and formation of soot which further determines the amount of heat released to the surrounding (Palacios Rosas 2011), flame stabilization (Wang et al. 2014), turbulence–chemistry interaction, and local extinction (Lyons 2007). Flame lift-off was defined as the separation distance of the visible flame and jet exit (Kalghatgi 1983; Bradley et al. 2016). A recent study by Zhou and Jiang (2016) using LSM stated that the inclusion of lift-off to determine the flame length could give variation in the total radiant heat release. From their study, it was observed that the horizontal release orientation gives a higher lift-off value than the vertical release (Zhou et al. 2016). This is due to the gravitational effect and viscous friction on the vertical orientation jet fire. The work implies that the flame length that includes the lift-off length may give a good estimation of radiant heat release as compared to that when the lift-off flame is excluded in the estimation. This study contradicts with the assumption made by Gómez-Mares et al. (2010) and Palacios et al. (2012) when using SFM in which the flame length is determined at the visible bottom to the top of the flame, excluding the lift-off. On the other hand, determination of point source in PSM and MPSM is based on the flame length that includes the lift-off length. Although many correlations include the lift-off distance as a function of velocity and burner exit diameter as listed in Table 3, one should be careful to reapply the correlations by taking into account the jet flame direction at first.
A previous study indicated that different burner diameters do not give a significant variation for flame lift-off; however, the value increases linearly with jet exit velocity (Kalghatgi 1983). As the jet velocity increases, more air will be entrained, and this could enhance the combustion process, by producing more premixed blue flame, leading to lifted flame. However, as stable flame length is reached, lift-off length will become increasingly sensitive to air entrainment (Kalghatgi 1983). The correlation proposed by Kalghatgi (1983) on this phenomena is as follows:
where G, ρj, Uj, and dj are the initial jet momentum flux, expanded jet density (kg m−3), expanded jet velocity (m/s), and expanded jet diameter (mm), respectively. A similar correlation has been applied to a work involving LPG horizontal jet fire issuing through 19 mm diameter nozzle at a velocity range of 25 to 210 m/s (Gopalaswami et al. 2016). Yet, this work gave an overprediction of lift-off length as compared to other previous studies using the same model (Suris et al. 1978; Sonju and Hustad 1984; Johnson et al. 1994; Santos and Costa 2005; Kiran and Mishra 2007; Palacios et al. 2009). It can be suggested that the lift-off length is highly sensitive to the threshold parameter in image processing analysis. Nonetheless, the dimensionless correlation was proposed based on the experimental dataset as
which is based on the primary equation that was first developed by Peter and Williams (1983) as per Eq. (30) when c is constant with a dimension of time (s)
However, Hu et al. (2013a) observed that the lift-off height is increased when the velocity increases on propane jet diffusion flame at a reduced atmosphere. From their work, the correlation at 64 and 100 kPa, respectively, has been developed
The result was in good agreement with the study done on vertical diffusion jet flame using propane as sample fuel from a circular nozzle between 4 and 6 mm diameter at the subatmospheric conditions of 60, 70, 80, and 90 kPa and normal atmospheric condition of 100 kPa (Wang et al. 2014). Palacios et al. (2016) observed in their work, for subsonic jet flame, a normalized lift-off distance which can be defined as
The data gathered by Bradley et al. (2016) has deduced the following equations for subsonic and sonic flame:
where f is the ratio of fuel to air moles in fuel–air mixture for maximum burning velocity and U* is the dimensionless flow number expressed as
where u, SL, d, δ, Pi, and Pa are the velocity (m/s), maximum laminar burning velocity of the mixture under ambient conditions (m/s), nozzle diameter, laminar flame thickness under ambient conditions (m), initial pressure, and ambient pressure, respectively. In the vertical direction, the lift-off may give a constant value at a point as the velocity increases. It can be explained by the gravitational force and a similar observation should be applied for horizontal orientation. Besides, the lift-off is dependent on the fuel type, by introducing the multiplying factor f as in Eqs. (33)–(35). From the discussion above, a summary of lift-off length correlation based on velocity, Froude number, and Reynolds number is summarized in Table 3.
Flame Width
In the literature, determination of radiant heat release was said to be closely related to flame length, shape, and lift-off length. There is a little attention given to the flame width which is directly linked to the flame shape configuration. It can be said that the flame width (W0) is proportional to flame length and approximately equal to 0.18 L (Mogi and Horiguchi 2009) for sonic hydrogen jet release in a horizontal orientation. Palacios and Casal (2011) investigated flame width from propane jet release in a vertical orientation at a different location along the flame length. It was found that flame width gives a better prediction at point of 0.7 L for both sonic and subsonic releases. Although flame width data are not usually included in the semi-empirical model, however, as an improvement made in LSM, the determination of flame width is equally important to flame length, shape, and lift-off. It was used to determine the average flame radius for flame emissivity calculation (Zhou and Jiang 2016; Zhou et al. 2016) and, consequently, the total amount of radiant heat released to the surrounding. In the case of flame impingement, the flame width may have a direct impact on the localized heat flux area. Since it was a function of velocity, thus, it can be said that the impinged area should be larger when jet release velocity is increasing.
Total Heat Release and Radiative Fraction
Other key parameters to be considered for radiant heat prediction are the total heat release and radiative fraction. It is especially important in PSM and MPSM models. Total power of combustion QT is a direct function of mass flow rate m (kg s−1) and net calorific value of the fuel H (kJ kg−1).
Radiative fraction η is defined as the ratio of total radiant heat emitted QR by the jet flame to the total heat release rate QT (Zhou et al. 2018). It is also defined as the amount of flame energy converted into escaping radiant energy. A normal way to obtain the η data is through experimental measurement for both QR and QT of the jet release.
The determination of the radiative fraction η is based on several factors such as fuel type, atmospheric condition, fuel flow rate, distance of measurement (near field and far field), geometry of fire, and fuel release conditions (velocity, temperature, and orientation) (Hankinson and Lowesmith 2012; Miller 2017). The applicability of η cannot simply be assumed. For example, if the η value is determined using the PSM model, similar η value should not be applied if one adopts the MPSM model in their heat release prediction. The situation is also applied to near- and far-field observations where η is determined in the far field from a jet fire, limiting the applicability to near-field observation (Hankinson and Lowesmith 2012).
An earlier study by Chamberlain (1987) correlates the radiative fraction with orifice exit velocity using natural gas as fuel in a vertical orientation.
where ueq is the effective exit gas velocity of the gas jet given by Birch et al. (1984)
where pj and p∞ are the absolute pressures at the jet exit pressure and in the atmosphere, respectively, while ρj is the jet exit density. Release flow from the jet exit forms an underexpanded jet and rapidly expands to ambient condition through a series of expansion shock (Schefer et al. 2006). The concept of the underexpanded jet is also known as a notional nozzle that has been explored by others (Birch et al. 1984; Schefer et al. 2006; Molina et al. 2007; Ekoto et al. 2014) as shown in Fig. 16. Effective diameter deff is introduced in this concept, on the basis of mass and momentum conservation equation (Molina et al. 2007), in which the value is often larger than the nozzle diameter.
From Fig. 16, level 1 indicates a high-pressure source (P1) with a temperature of (T1); level 2 is the jet exit with release diameter, pressure, temperature, and velocity of (d2, P2, T2, v2), while level 3 is the ambient condition where the jet expands to temperature, pressure, and velocity of (T2, P2, v2). It is assumed that the velocity is uniform at level 3 and usually at sonic condition. Another assumption is made which includes that there is no air entrainment between levels 2 and 3 (Molkov and Saffers 2013). The diameter of deff is usually larger than the jet exit diameter, d2. In this particular case, the η value drops with the increase of jet velocity due to improved combustion quality with the lower portion of the jet beginning to become blue at larger jet velocity (Kiran and Mishra 2007; Zhou and Jiang 2016).
Markstein and Ris (1990) have carried out experiments on the radiative fraction against total heat release and correlated radiative fraction to global residence time, derived from a convective timescale. Molina et al. (2007) coupled global residence time to correction factor; however, the application is limited to nonsooting flame such as hydrogen in the momentum-controlled regime. Radiative fraction value is dependent on the fuel type and its reactivity, which will determine the combustion quality. The combustion quality and its associated heat release can be correlated to its carbon content and type of bonds, i.e., alkanes, alkenes, and alkynes. There are numerous studies that have been conducted to compare the combustion quality and fraction of heat radiated by different types of carbon number (Lowesmith et al. 2007). The fuels include butane, propane, natural gas, crude oil, and butane/natural gas mixtures. For hydrocarbon with higher carbon content, more soot is produced with higher emission and, thus, induced more heat radiated (American Petroleum Institute 2008). From the work of Hankinson et al. (2007), they suggested that the radiative fraction was 0.13 for natural gas, 0.24 for propane, 0.32 for butane, and 0.5 for crude oil. For the mixtures of butane/natural gas, the radiative fraction is directly proportionated with butane content; when the content of butane in mixtures increases, the fraction of heat-radiated η would also increase.
The work of Lowesmith and Hankinson (2012) reported that fuel mixtures are dependent on the carbon content of the individual component that contributes to the highest percentage of total mass. For liquid–gas mixtures, η can be estimated by using the following equation as proposed by Lowesmith et al. (2007):
where ηm is the fraction of heat radiated of the mixture, x is the mass percentage, ηL is the fraction of heat radiated of liquid, and ηG is the fraction of heat radiated of gas. Studer et al. (2009) have conducted a study of large-scale methane/hydrogen jet fire and found that when the methane content (%) increases in the mixture, the fraction of heat radiated would also increase as depicted in Fig. 17.
Based on the work reported by Lowesmith et al. (2007) on the fraction of heat radiated and the relation to field of observation, it can be said that PSM is not suitable to be used at a near distance (within one flame length) and this gives an advantage for SFM to be adopted on heat release prediction. If one used PSM for measurement of incident radiation data in the near field, the correction factor is needed to apply in order to obtain the correct fraction of heat radiated or otherwise use the weighed MPSM approach. The effects of near field and far field on the fraction of heat-radiated measurement have been extensively explored by Hankinson and Lowesmith (2012) using various modeling approaches that include SFM, PSM, and MPSM. From their findings, the PSM approach may provide erroneous results for a radiative fraction if incident radiation data (QR) in the near field is used. Meanwhile, the use of MPSM shows better agreement with near-field observation. Figure 18a–f shows the prediction models in near-field observation as a function of normalized distance along the flame axis and the comparison between the experimental data from Sivathanu and Gore (1993) and Baillie et al. (1998). From the figures, it can be seen that the normalized incident radiation (Cx = Qmeas/Qmodel) of selected models is based on the single-point source model using distance R (refer to Fig. 4), called PSMR.
Figure 18a shows the prediction value of Cx at a radial distance of 0.5 L and varying axial location using Qmeas of MPSM, Fig. 18b using Qmeas of PSM with distance S, Fig. 18c using Qmeas of SFM with cylinder shape, Fig. 18d using Qmeas of SFM with cone shape, Fig. 18e using Qmeas of SFM with back-to-back cone shape, and Fig. 18f using Qmeas of SFM with back-to-back ellipsoid.
It can be clearly seen on Fig. 18a that the predicted value of CxMPSM/PSMR peak is in the correct region in the axial direction and the curve lies within the bounds of the data presented by Sivathanu and Gore (1993), while Fig. 18b shows the overpredicted value of Cx and the peak obtained was slightly off to the left when compared with the experimental data values, implying poor agreement with the data when using PSM prediction. Figure 18c use an assumption of cylindrical shape when prediction using SFM is adopted, and it shows an overpredicted value and earlier peak detected at lower radial distance. SFM with conical shape shows slightly better agreement than when the cylinder shape is used as illustrated in Fig. 18d. In Fig. 18e–f, when using SFM with back-to-back cone and ellipsoidal shape, respectively, it shows agreeable data in terms of shape and peak location. From the comprehensive comparison between model prediction and experimental data, it can be concluded that MPSM offers a better approach for radiant heat prediction in the near field, and PSM is unsuitable for near-field observation, while SFM is suitable if the correct flame shape is used to represent the flame configuration.
Other than that, jet fire orientation also holds considerable effects on the radiative fraction as indicated by Zhou et al. (2016). In their study, they have correlated Froude number to radiant heat fraction. However, there is no physical interpretation in detail.
In general, most of the correlations for radiative fraction are not valid to low luminosity gases such as hydrogen and syngas mixtures (Miller 2017). Thus, a series of experiments have been conducted using hydrogen and syngas as fuel in a vertical and horizontal orientation. The model developed in the study called AP flame adopted the MPSM approach to determine the total heat radiating from the flame, in which it is distributed as individual point sources along the flame centerline, weighted to be maximum at the widest point of the flame, about two thirds along the flame as illustrated in Fig. 19.
Total heat radiating from the flame QR is determined using radiant heat fraction η from the Chamberlain correlation and it was found to be reasonable for the natural gas jet flame in a vertical and horizontal orientation. For hydrogen jet fire, the radiant heat fraction is correlated to mass flux at pipe exit, Mflux. The data is found to be well fitted for vertical hydrogen jet fire, but the value is higher for equivalent horizontal and 45° release hydrogen flames. This phenomenon occurs probably due to the reflection of thermal radiation off the ground between the flame and the point of measurement and/or the hot ground underneath the flame preheating some of the air entering the flame, increasing the flame temperature, and would diminish once the flame is elevated higher off the ground. In this case, a correction factor was applied where the equation is given as
where ηH is the radiant heat fraction in a horizontal orientation, ηV is the radiant heat fraction in a vertical orientation, Lc is the centerline flame length, and hRC is the distance between the flame radiant center and the ground. For hydrogen/natural gas mixture jet fire, the η was found to be similar for 45° and horizontal jet flames at the same flow rates, while for the mixtures with the presence of an inert, radiative fraction, η increased as the content of inert increases (Fig. 20).
Later, a completely new dimensionless group has been introduced in generalizing the radiative fraction correlation, consisting of the flame Froude number, mass fraction of fuel at stoichiometric conditions, and the density ratio of fuel gas to ambient air to a radiative fraction (Zhou et al. 2018). The study covers hundreds of orifice exit diameters using a range of fuels (hydrogen, methane, and propane) at vertical and horizontal orientations, buoyancy- and momentum-dominated releases, and subsonic, sonic, and supersonic velocities. It was found that the capability exceeds previous correlation based on Froude number only or the global residence time with/without correction factors. The equation deduced from the theoretical analysis of the radiative fraction and yield is as follows
where η, fs, ρs, and ρ∞ are the radiant heat fraction, mass fraction of fuel at stoichiometric condition, gas density at the jet exit, and ambient air density, respectively. It must be noted again, in the semi-empirical models, that η is only accounted in PSM and MPSM. Meanwhile, for SFM and LSM, the radiative heat was assumed to totally depend on the flame shape configuration.
Atmospheric Conditions
The dispersion behavior of fuel released heavily depends on atmospheric conditions. This includes the wind speed, wind direction, ambient temperature, relative humidity, and ambient pressure. An experiment conducted by Hu et al. (2013b) on vertical propane jet fire characteristics in a reduced atmospheric pressure depicted that the mean flame height is higher in subatmospheric conditions as well as the flame lift-off height. This condition can be correlated to a fraction of stoichiometric air entrained, na, a basic parameter in the flame height correlation.
In their work, they prescribed, in normal atmospheric pressure, the value of n = 9.6; however, the value is 73% lower for subatmospheric pressure condition. The change of atmospheric pressure may have a direct effect on the flame height and lift-off height, giving higher value in reduced atmospheric pressure (Hu et al. 2013a). However, none of the models have ever considered the change of pressure as most of the jet fire occurrence was assumed to occur at normal atmospheric pressure. On another note, wind speed and wind direction are also held to have considerable effects on the jet fire characteristics particularly on flame shape and appearance as well as the heat distribution to the surrounding. This indirectly gives variation to the fraction of heat radiated η (Gómez-Mares et al. 2010). In a study conducted by Huang et al. (2017), wind speed can be correlated to the maximum flame width of jet flame geometrical properties. Clearly, it can be said that wind speed and direction give a direct effect to flame geometrical features, consequently the fraction of heat radiated to the surrounding in the case of free jet fire occurrence and thermal distribution to the surface impinged in the case of jet flame impingement.
All models, i.e., SFM, PSM, MPSM, and LSM, agreed that atmospheric transmissivity τ value also is very important. As can be seen from Eq. (44), each model takes into account atmospheric transmissivity (τ) due to the absorbance of radiant heat through atmosphere intervention as it goes to the local recipient in every jet fire occasion (van der Bosch et al. 2005). It was a function of ambient temperature and relative humidity. The value was normally taken close to unity. It implies that the total heat released by the jet fire is not best representing heat received by the recipient and this would give an under- or overprediction on the total radiative heat to the receivers. van der Bosch et al. (2005) highlighted a method to determine the atmospheric transmissivity (τ) as
where αw is the water vapor absorption factor and αc is the carbon dioxide absorption factor. Detailed calculation of water vapor absorption factor, αw, and carbon dioxide absorption factor, αc, has been detailed elsewhere (van der Bosch et al. 2005). Since water vapor and carbon dioxide are a major constituent in radiant heat wavelength that would reduce the absorption factor to be less than unity, thus the observation field plays some significant roles in the determination of the transmissivity value. The assumption might be true for measurement of distance at a small distance. However, it may provide an erroneous measurement at the far field. This is due to absorptivity of the radiative wave through major constituents of combustion products, carbon dioxide and water vapor; thus, it shall not be ignored particularly for far-field measurement.
On the other hand, atmospheric transmissivity value also can be expressed as a direct function of relative humidity, RH, and distance from the flame surface to the receiver, X, as mentioned elsewhere (Brzustowski et al. 1975; Palacios et al. 2012):
However, atmospheric transmissivity values available in the literature are generally different with the values given by research works. For example, the study performed by Hankinson and Lowesmith (2012) depicted that the value of τ depends on prevailing atmospheric conditions (temperature and humidity) as it is largely driven by carbon dioxide and water vapor in the atmosphere (Kohout and Turpin 2013). Some other studies made an assumption that the transmissivity term should be unity or close to unity (Gómez-Mares et al. 2010; Zhang et al. 2015). It was suggested that the value is taken as unity when the distance relative to the heat source is less than 10 m (UKOOA 2006). Another method that can be used to estimate the values of τ is by using equations found in Rohsenow et al. (1998). This method was applied by Gómez-Mares et al. (2010) for a mass flow rate of 0.09–0.43 kg s−1 of propane, applying an SFM to obtain QR, and the estimated uncertainty is ± 3% with 95% confidence level. However, the data of QR are scattered relative to the distance where the measurement is taken. This is due to the turbulence phenomenon and flame oscillation in far-field observations which has a direct influence on the sensor measured (Gómez-Mares et al. 2010). Sonju and Hustad (1984) reported quite a scattering results with 60% variation, higher than the variation obtained by Gómez-Mares et al. (2010).
It is interesting to note that the study of Molina et al. (2007) did not take into account the atmospheric transmissivity term for large-scale jet fires when the PSM was applied in their work. The absence of the τ term led to quite significant differences in predicting the radiation value due to the fact that the energy is absorbed by the atmosphere at larger distance measurement. Later, it was found that the term could only be omitted at smaller distances (say, less than 3 m), where it was typically used in the experimental setup. From the experimental point of view, it was found that less radiant energy is lost to the atmosphere; thus, the transmissivity value is nearly unity (Hankinson and Lowesmith 2012). A work done by Mousavi and Parvini (2016) on the study of effective factors on leakage-induced hydrogen jet fire found a large variation in radiation heat measurement and suspected that leakage diameter, release pressure, and release height are the contributing parameters as compared to humidity and ambient temperature which have less significant effect. However, it is advisable to be careful when applying the transmissivity term to estimate the radiation heat at the larger-scale jet fire or measurement taken from far-field observation (Molina et al. 2007). An abnormal atmospheric condition in terms of relative humidity should also be taken into account as it poses a possible deviation from the true measurement of incident radiation. As a summary, it can be said that consideration of atmospheric transmissivity is independent relative to the type of model used but largely driven by the relative distance of the recipient.
Conclusion and Future Direction
This review has highlighted the governing parameters to determine radiant heat intensity from various jet release scenarios, different orientations, and scale of release and how the predictive models consider the important parameter in their model in order to give reliable and realistic results. The state of our knowledge about semi-empirical models used to estimate radiation heat from jet fire phenomena as revealed in this review suggests that there is still a long way to go before we can predict with any confidence. The following conclusions and future directions can be drawn from the analysis:
-
(i)
No general quantitative model is available to best predict the heat radiation from the jet fire in near- or far-field scenarios. This is hindered by several factors: (a) scale of the jet fire (small, medium, large), (b) distance from which the measurement is taken (near and far field), (c) jet fire orientation, and (d) other external factors such as geographical conditions.
-
(ii)
For radiation estimation within a near-field observation, estimation given by the SFM and LSM appears to be more realistic as they consider the flame shape orientation and, hence, it provides better emissivity value. In general, cylindrical shape is the most common shape used to represent the flame shape in a vertical orientation, while other studies suggested rectangle and kite shapes to best represent the flame shape in a horizontal orientation. It was also found that the combination of flame shape has received little consideration although it could give a good approximation of flame surface. Thus, in a newly developed model LSM, a combination of flame shape has been studied and it was found that kite shape with the inclusion of lift-off best represents the flame shape for medium-scale jet flame in a horizontal orientation. However, more data is needed to close its application for small- and large-scale jet flame. For vertical jet fire, it was found that back-to-back cone fits the small jet flame and the combination of cone in the lower region and of cylinder in the upper region fits relatively the large-scale jet flame. It is also suggested to include the effects of flame with low luminosity such as hydrogen to the applicability of LSM.
-
(iii)
There are two common types of MPSM: weighted MPSM and simple MPSM. In the near-field observation, weighted MPSM is more suitable to be used as compared to simple MPSM for jet fire in a vertical orientation, while in the far-field observation, the behavior of the weighted MPSM approximate to PSM indicates that weighted MPSM is suitable for both near- and far-field observations.
-
(iv)
Due to the deformation of jet flame that can be caused by external factors such as wind speed, it resulted in an underestimation of radiant heat release up to 40%. Thus, consideration of the buoyancy region has been taken care of with the suggested method of the 1D flame integral model and the AP flame model. For jet flame with only buoyancy-dominated region, the projected length LP should be measured as a function of nozzle width.
-
(v)
The PSM is more suitable to be used in far-field observation and the MPSM seems to give a realistic value considering the jet fire with buoyancy effects.
-
(vi)
Although LSM is a newly developed model, the prediction of radiant heat gives encouraging result relative to the validity of the model system. It does yield the expected values not only for near-field but also for far-field incident radiation, making this model usable in all practical situations. However, the challenge of using this model is that more data is required to ensure the validity and wider application for different fire orientations and scales.
Abbreviations
- A IR :
-
2D area of the flame surface
- c 2 :
-
Constant parameter cp specific heat of air at constant pressure (kJ kg-1 K-1)
- c p :
-
Specific heat of air at constant pressure (kJ kg-1 K-1)
- C x :
-
Normalized incident radiation (qmeas/qmodel)
- D eq :
-
Equivalent diameter of flame
- d :
-
Diameter of nozzle exit (mm)
- d eff :
-
Effective diameter
- d j :
-
Expanded jet diameter
- E :
-
Flame emissive power per area (kW m−2)
- Fr :
-
Froude number
- f :
-
Multiplying factor
- f s :
-
Mass fraction of fuel at stoichiometric condition
- G :
-
Initial jet momentum flux
- h RC :
-
Distance between the flame radiant center and the ground
- H :
-
Net calorific value of fuel (kJ kg−1)
- L :
-
Flame length from orifice (m)
- L 0 :
-
Flame length with zero wind
- L b :
-
Flame length in buoyancy region
- L c :
-
Centerline flame length
- L f :
-
Lift-off distance (m)
- L IR :
-
Radiant flame length
- L m :
-
Flame length in momentum region
- L n :
-
Nozzle length
- L p :
-
Projection distance
- m :
-
Mass flow rate (kg s−1)
- n a :
-
Stoichiometric air entrained
- n(N):
-
(Total) number of point sources
- P a :
-
Ambient pressure
- P i :
-
Initial pressure
- P 0 :
-
Stagnation pressure
- P out :
-
Pressure downstream of jet fire
- Q :
-
Heat release rate (kW)
- Q R :
-
Incident radiation
- Q s * :
-
Dimensionless heat release rate
- \( {Q}_{\zeta_{\mathrm{l}}}^{\ast } \) :
-
Dimensionless heat release rate as defined in Eq. (19)
- Q T :
-
Net power of the flame (kW)
- r(r 0):
-
(Maximum) flame radius (m)
- R :
-
Distance perpendicular to flame axis (m)
- Re :
-
Reynolds number
- RH:
-
Relative humidity of atmosphere (%)
- S :
-
Distance from a point within the flame to the receiver (m)
- S L :
-
Maximum laminar burning velocity of the mixture under ambient conditions (m s−1)
- T :
-
Temperature
- T ∞ :
-
Ambient air temperature
- \( \overline{T_{\mathrm{f},\mathrm{a}}} \) :
-
Mean flame temperature rise
- u :
-
Velocity (m s−1)
- u eq :
-
Effective exit gas velocity of the gas jet
- U * :
-
dimensionless flow number
- u j :
-
Expanded jet velocity (m s−1)
- V :
-
View factor
- W o :
-
Flame width
- W n :
-
Nozzle width
- x :
-
Mass percentage
- X :
-
Distance from the flame surface to exposed target (m)
- EPPLL:
-
Emissive power per line length
- LSM:
-
Line source model
- MPSM:
-
Multipoint source model
- PSM:
-
Single-point source model
- SFM:
-
Solid flame model
- α :
-
Length ratio of lower flame to the whole flame
- α t :
-
Tilt angle
- α w :
-
Absorption factors (water vapor)
- α c :
-
Absorption factors (carbon dioxide)
- δ :
-
Lift angle
- δ f :
-
Laminar flame thickness under ambient conditions (m)
- ε :
-
Flame emissivity
- σ :
-
Stefan–Boltzmann constant (5.67 × 10−8 W m−2 K−4)
- η :
-
Fraction of heat radiated
- η H :
-
Fraction of heat radiated in a horizontal orientation
- η m :
-
Fraction of heat radiated of mixture
- η G :
-
Fraction of heat radiated of gas
- η L :
-
Fraction of heat radiated of liquid
- η V :
-
Fraction of heat radiated in a vertical orientation
- τ :
-
Atmospheric transmissivity
- θ :
-
Angle as shown in Fig. 4
- φ :
-
Angle as shown in Fig. 4
- ρ j :
-
Expanded jet density (kg m−3)
- ρ s :
-
Gas density at the jet exit
- ρ ∞ :
-
Ambient gas density
- γ :
-
Ratio of specific heats
- ξ :
-
Richardson number
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Funding
The authors would like to express their appreciation for the support of the sponsors—Research University Grant (GUP) [Grant Number = Q.J130000.2546.17H82: Parametric and Thermal Investigation of Horizontal Buoyant Jet Fires Impingement Radiation on Plant Installation].
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Ab Aziz, N.S., Md. Kasmani, R., Samsudin, M.D.M. et al. Comparative Analysis on Semi-empirical Models of Jet Fire for Radiant Heat Estimation. Process Integr Optim Sustain 3, 285–305 (2019). https://doi.org/10.1007/s41660-019-00081-y
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DOI: https://doi.org/10.1007/s41660-019-00081-y