Abstract
The paper presents the variability of hard coal output, methane content and methane emissions into coal workings and into the atmosphere from the two most methane-gassy coal mines in Poland. The Budryk mine is one of the youngest mines in Poland, but it is the most methane-gassy as well. In 2016, the total CH4 emissions exceed 140 million of m3. This large increase in methane emissions to mine workings is primarily related to the increase in the depth of coal extraction (up to 1290 m) and, consequently, the rapid increase in the methane content in coal seams (up to 10–12 m3/Mg coaldaf). On the other hand, in the Pniówek mine, methane emission was the highest at the beginning of the study period (1986–1991). During the following years, emission decreased to the values of less than 140 million of m3, which were still one of the largest amounts of emitted methane in the entire Upper Silesian Coal Basin. The coexistence of natural factors, such as the geological structure and gas distribution, as well as mining-related factors, i.e. the depth of mining, the intensity of coal extraction determines the temporal variability of methane emissions in the studied mines.
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Introduction
The Upper Silesian Coal Basin (USCB) (Fig. 1) is the most industrialised region in Poland, providing bituminous coal for heat and power generation, as well as coking coal for coke production. Reaching deeper deposited coal seams carries a high methane risk, a risk of underground tremors, and intensification of temperature hazards. The increase of methane emission is one of the most dangerous problems in modern mining activity and entails work suspension, evacuations and even fatalities after methane explosions (Trenczek 2016; Duda and Krzemień 2018; Dreger and Kędzior 2019). Two mines from the USCB, Budryk and Pniówek—members of the Jastrzębska Spółka Węglowa SA, were chosen to identify and study variations in methane emissions. These two mines are characterised by the highest CH4 emission in the entire coal basin in Poland. Methane emissions to coal workings in the studied mines are often more than 100% higher than in other mines in the basin (GIG 1995–2019). The total methane emission in the USCB has been changing with time. In 2004, methane emission from all mines amounted to more than 800 million m3 and in 2015 exceeded 900 million m3. The entire emission values fluctuated from year to year, but the overall emission trend is increasing. A similar trend was observed in other coal basins, where coal was extracted from deeper levels every year e.g. (Ju et al. 2016; Wang et al. 2019; Karacan and Warwick 2019). On the other hand, the hard coal output in Poland has been constantly decreasing from over 100 million Mg at the end of the twentieth century to around 60 million Mg in 2016–2018. Methane (CH4) is the second-most important greenhouse gas after the notorious carbon dioxide (CO2) and plays a potent role in atmospheric chemistry and radiation balance (Warmuziński 2008; Ghosh et al. 2015; Kędzior 2015; Tutak and Brodny 2019; Swolkień 2020; Dreger 2021).
The amount of methane emission from a coal deposit is strictly dependent on many factors, which can be roughly divided into natural factors related to the geological structure of the deposit and its natural gas content and pressure, as well as anthropogenic causes resulting from mining activities and the method of deposit exploitation e.g. (Karacan et al. 2011; Krause and Smoliński 2013; Kędzior and Dreger 2019; Dreger 2020). Therefore, the interrelationship of available results regarding the gas content of the deposit, volume and intensity of coal extraction with the data on the quantity of methane emissions should make us aware of how strongly the described factors affect the phenomenon of emissions and, therefore, how to counteract it.
Accordingly, the main purpose of this article is to show how the dependencies and causes of methane emission and hard coal output have changed with time (1986–2018) in the two most methane-gassy coal mines in Poland. The Pniówek coal mine is characterised by the one of the highest methane emissions in Poland. In the Budryk mine, methane emission has been increasing rapidly since 2013 and now it is the highest in the country.
Data sources
All the data were obtained from officially accepted geological documentation from the Budryk and Pniówek mines belonging to the Jastrzębska Spółka Węglowa SA (JSW—internal reports). In addition data from the Annual Report (for the years 1994–2018) on the state of basic natural and technical hazards in the hard coal mining industry published by the Central Mining Institute (GIG) in Katowice (GIG 1995–2019) were taken for calculations and analyses.
The most important data taken into research are the methane emission from two selected underground coal mines—Budryk and Pniówek. The total methane emission (CMM—coal mine methane) refers to methane liberated from the coal and surrounding rock strata due to mining activities. It is a combination of ventilation air methane (VAM) and methane coming from coal seam drainage (degassing). Ventilation air methane and degassing were also studied for these two coal mines. The VAM is commonly determined by measuring the pure methane concentration in the air stream by handheld anemometer and by taking air samples to the laboratory tests. The air velocity measurements are important to determine the methane concentration in the return airways (e.g. Karacan et al. 2011; Gawlik and Grzybek 2002). The specific CH4 emission was investigated as well. This feature describes how many methane is emitted to the mining atmosphere with every extracted Mg of coal and it shows the real methane danger during mining activities. To measure the amount of adsorbed CH4 in coal, we use the term methane content, which describes the volume of gas in one Mg of coaldaf (daf is the pure coal substance, without moisture and ash, dry ash free coal substance) (Wierzbicki and Skoczylas 2014; Honysz 2015).
Moreover, to study relations between methane content and coal seam pressure (methane desorption), the data collected by Tarnowski (1971) and CLP-B Sp. z o.o. Laboratory in Jastrzębie-Zdrój were also considered and carefully analysed. After the analysis of all collected data, the multi-criteria geology and mining evaluation were set up.
Coal mines under study
Budryk mine
The Budryk coal deposit is located in the northern part of the basin (Fig. 1) at the north-western flank of the Main Trough between two dislocations: the Kłodnica Fault in the north and the Bełk Fault in the south. The Budryk deposit is composed of 43 documented coal seams (from 325 to 407/3), all of which are found in the Orzesze, Załęże and Ruda beds. The deposit has a diverse geological structure, sediment disorders, and large tectonic variability (Table 1, Fig. 2). Carboniferous top surface varies in depth from + 60 m in the north to + 300 m above sea level in the south-east. The dip of the beds is varied, from almost horizontal to incline at 15° angle.
The largest dislocations in the USCB, such as the Kłodnica, Książ or Bełk faults, have nearly latitudinal orientation and displace layers to the south (Kędzior et al. 2013; Dreger and Kędzior 2019).
The Budryk mining area is represented by the Pennsylvanian Upper Silesian Sandstone Series (Namurian C; Serpukhovian and Bashkirian) and the Mudstone Series (Westphalian A and B; Bashkirian) (Table 2). In the profile of documented coal deposit Ruda (Namurian C; Bashkirian), Orzesze and Załęże (Westphalian B; Bashkirian) Beds were found.
The Upper Silesian Sandstone Series is represented by Ruda Beds occurring below the 407 seam where coarse and fine-grained sandstones were found. The following Załęże and Orzesze Beds (Westphalian A and B; Bashkirian) occur in all of the area with 800–1250 m thickness in total. They constitute the main stratigraphic unit in the deposit, built of mudstones, claystones and sandstones, with numerous coal seams which are the subject of mining.
Most of the Orzesze strata and the entire Carboniferous younger series (Cracow Sandstone Series) were removed by erosion in the mine area under study.
The overburden rocks lie discordantly on the Carboniferous erosion surface and consist of Triassic sandstones and carbonates, Miocene clays, as well as fluvial and glacial sediments of Quaternary origin. The total thickness of the overburden strata does not exceed 200 m (Table 3).
Pniówek mine
The Pniówek coal deposit is located in the south-western part of the USCB (Fig. 1) at the SW limb of the Main Trough, bordering with the Bzie-Czechowice fault zone in the south. The Pniówek coal deposit is a multilayer structure consisting of 62 documented seams of various thicknesses and qualities of the beds. Tectonic character of the deposit is also very complex, with fault throws between 10 and 300 m (Table 1, Fig. 3). Furthermore, we can distinguish many smaller faults accompanying larger dislocations throwing down the layers by a few metres.
The lithological profile of the Carboniferous strata within the discussed mine comprises the Pennsylvanian Paralic (Namurian A; Serpukhovian, Bashkirian), Upper Silesian Sandstone (Namurian B and C, Bashkirian), and Mudstone (Westphalian A and B; Bashkirian) Series.
All the Upper Carboniferous series are represented by clastic rocks, i.e. sandstones, mudstones and claystones in various quantitative proportions with numerous coal seams.
The Carboniferous top surface displays an erosive character and is morphologically varied. There are many paleo-ridges and washouts with a general NW orientation. There are clay and sandy Miocene deposits on the eroded Carboniferous surface. Their thickness is variable and ranges from about 200 m in the north to 1000 m in the south (Table 3).
Results and discussion
Methane distribution
Budryk mine
Current spatial distribution of the methane content in the Upper Silesian Coal Basin depends inter alia on the geological development of the basin in the past, the sorption capacity of the coal seams, the thick and hermetic Miocene overburden (methane accumulation), lithological character of Carboniferous sediments, and tectonic dislocations (methane migration) (Kozłowski and Grębski 1982; Kotas 1994; Kędzior 2009a, 2019; Słoczyński and Drozd 2018; Krause 2019) (Figs. 2, 3). In the Upper Silesian Coal Basin, two main geological patterns of vertical distribution of coal-bed methane (CBM) were distinguished (Kotas 1994; Kędzior 2009a) (Fig. 4). Pattern A is associated with northern and central areas of the coal basin, characterised by the presence of naturally degassed coal seams down to the depth of 400–600 m or deeper in some areas. With depths greater than 500 m, the CH4 content increases rapidly until it reaches the primary methane zone with methane content of up to 15 m3/Mg coaldaf. Going deeper, methane content tends to decrease. The northern pattern (A) is related to the Budryk mine, which is located in the north-western part of the basin (Fig. 1). Figure 4a illustrates the distribution of methane content in the Budryk coal seams (JSW—internal reports).The natural degassed zone is evident to the depth of 600 m, then methane content increases rapidly until the primary zone of methane content is reached. It is evident here, that thin and permeable Triassic and Miocene overburden is not sufficient to stop the migration of gases upwards (Table 3). The average and maximum CH4 content in the Budryk seams tend to increase with depth, reaching maximum values of over 7 (average) and 15 (maximum) m3/Mg coaldaf between − 750 and − 990 m above sea level (between ca. 1000 and 1200 m below ground level). (Fig. 4). The depth range of the primary methane zone has not been exactly determined so far in the mine under study.
Figure 2 shows the fault distribution in the Budryk mine field (402 coal seam). These dislocations form a dense network of faults with latitudinal (Barbara fault zone) and longitudinal (e.g. Knurów and Chudecki faults) orientation (Table 1). The existing fault network probably aided the natural process of degassing the upper parts of the deposit in the geological past, and the faults themselves may today constitute the boundaries between the deposit parts with different level of gas saturation, and thus have different effects on the intensity of gas emissions to the mine workings of the Budryk mine. The role of faults in gas migration has also been studied elsewhere (e.g. Thielemann et al. 2001; Karacan and Olea 2014; Karacan et al. 2021).
Pniówek mine
Pattern B is associated with the southern part of the basin and includes two distinct zones of methane content (Fig. 4b). The first methane zone covers the secondary accumulation of CH4 adsorbed in coal seams and free gas accumulated immediately below the thick and impermeable Miocene cover (Fig. 4b). The next methane zone, so called primary with increased concentrations of methane is separated by an interval of reduced CH4 content in coal seams (400–800 m below ground level, Fig. 4b). The primary methane zone lies deeper (> 1000 m), with the CH4 content of up to 10–16 m3/Mg coaldaf (Kotas 1994; Kędzior 2012). This zone contains thermogenic methane produced as a result of the coalification process in the late Carboniferous period (Kotarba 2001). Increased methane content in the uppermost part of Carboniferous coal-bearing series sealed with hermetic overburden is conditioned by the occurrence of microbial methane produced in the pre-Miocene period and then mixed with thermogenic methane (Kotarba and Pluta 2009; Kędzior 2019). The methane depth zones with faults in the area of the Pniówek mine are shown in Fig. 3. The main dislocation of Bzie-Czechowice, which is a regional dislocation in the basin scale, is located in the south of the studied area and displaces the primary gas-bearing zone in the throw direction (to the south, Fig. 3). Together with the remaining faults (e.g. Krzyżowice I and II), they seem to be migration pathways for gas between the primary and secondary methane zones. Probably thanks to them, thermogenic methane migrated towards the Carboniferous top and supplied the secondary gas-bearing zone (Kędzior 2009a, 2012).
The pressure of gas accumulated just below the Miocene cover is higher in comparison to the remaining parts of the Carboniferous series and oscillates around 6–7 MPa (Tarnowski 1971). After the Carboniferous period (especially in Mesozoic and Paleogene time), the top surface of coal-bearing formations were exposed and subjected to weathered and erosion processes. To the present, in the topmost part of the Pniówek coal deposit, a layer of coal-bearing detritus with a high 20–30% porosity has been preserved and now is sealed by the Miocene deposits. The currently observed zone of increased gas pressure is associated with porous coal-bearing weathered deposits in the Carboniferous top (Janas 1962; Tarnowski 1989), which is a reservoir of both secondary microbial gas and migrating thermogenic methane (Kotarba and Pluta 2009).
The differential vertical and horizontal methane distribution in coal basin caused by e.g. overburden occurrence, faulting and folding was identified in many coal basins (Ju et al. 2016; Diamond 1994; Noack 1998; Thielemann et al. 2001). The Pniówek mine corresponds to the southern pattern of the CH4 vertical distribution (Fig. 4b). In contrast to the Budryk mine, the thick and impermeable Miocene Skawina Formation (Table 3) has prevented gases release from coal seams to the atmosphere in the geological past. A comparative description of the Carboniferous series overburden in both described mines is presented in Table 3.
Methane content vs. pressure and sorption capacity
The volume of adsorbed methane, in the same temperature and pressure conditions, depends on micropores and macropores content in coal. Kozłowski and Grębski (1982) showed that more microporous coals can accumulate more methane in the coal structure. Studies carried out on coals from Western Canada (Lamberson and Bustin 1993) revealed that vitrinite-rich coals have a greater sorption capacity than inertinite-rich colas in the same rank, however research from the 1970s (Harris and Yust 1976) displayed that coal micropores are predominantly located in vitrinite, while in the inertinite, meso- and macropores. Moreover, the temperature and moisture have a negative influence on the sorption capacity of coal (Kozłowski and Grębski 1982; Kędzior 2009b, 2019; Wierzbicki 2013). The gas (methane) pressure in the coal seam is determined by the methane content in coal (Tarnowski 1989, 1971; Lunarzewski 1998) and is defined by the desorption intensity. This method is commonly used in the Polish and worldwide mining industry (Kozłowski and Grębski 1982; Lama and Bodziony 1998; Wierzbicki and Skoczylas 2014; Krause 2019) to classify the methane danger, before the more accurate tests will be carried out by the certified mining laboratories. The collected data of the gas pressure, in the southern part of the Upper Silesian Coal Basin by Tarnowski (1971) revealed that methane content in the coal seam is fairly correlated with the methane pressure/desorption intensity (Fig. 5). The recent results of tests made by the CLP-B Sp. z o.o. in Jastrzębie-Zdrój (Poland) for the Budryk and Pniówek mines for the years 2018–2020 showed similar outcomes describing the methane content and gas desorption/pressure interdependence (Fig. 6a, b).
Coal mining
The most important economic factor in every mine is the annual coal production. Economic possibilities, natural hazards, technical difficulties and market size affect the annual coal output of each mine (Dreger 2019, 2020; Dreger and Kędzior 2019). Changes in coal production over time in both analysed mines are illustrated in Fig. 7.
The Budryk mine started production in 1994, while the production data from Pniówek starts from 1986. In 1994, the Budryk mine was getting started with just 580 thousand Mg of extracted coal (Fig. 7). Over the following years, coal production in Budryk was gradually increasing, reaching the highest production level in 2007 with 3.85 million Mg of extracted coal. In subsequent years, until the end of the study period, coal output dropped and retained a constant level of under 3 million Mg per year.
On the other hand, the highest hard coal output in Pniówek was reported at the beginning of the research period, in the late 1980s, with the coal production exceeding 3.8 million Mg. In the next years, to the end of the studies, the coal production fluctuated which can be seen on Fig. 7.
Hard coal extraction in Polish underground mining is deeper about 8 m per year on average (GIG 1995–2019). As a result, coal production takes place in coal seams of variable gas and physico-chemical conditions. In most mines, in the USCB, methane content increases with increasing depth (Kędzior and Dreger 2019; Krause 2019). As the depth of extraction increases, gas permeability in coal seams decreases and pre-mining methane drainage is not sufficient; therefore, the methane hazard increases. The average depth of coal extraction in 2010 was around 700 m, and from year to year it was permanently increasing by 8–10 m. Now, the average depth of coal production is 788 m and coal sorption capacity is much lower than in shallower seams and the gas pressure in coal seams increases with depth (GIG 1995–2019; Kotas 1995; Krause 2019; Szlązak et al. 2020). Studies conducted by Krause (2019), e.g. revealed that most of the methane emitted to the coal workings comes from depleted, overlying and underlying coal seams (60%), the remainder of CH4 is emitted from extracting longwall (40%). Another important factor is the intensity of coal production. Hard coal in the USCB is almost exclusively produced by means of longwall systems with the use of heading machines and longwall mechanical coal miners (Krawczyk 2020). Longwall length and height, daily extraction progress are the main variables needed to determine the amount of the coal output. The longwall length increased by ~ 41% in recent years, coal production intensity rose and total methane emission also increased (Turek 2007; Krause 2019). As longwall length increases, the area of exploitation relaxation rises and the volume of released and migrated methane is also higher.
In the Budryk mine, with the greatest depth of mining in the USCB, currently reaching 1290 m, the number of operating walls has been changing during the studied period of coal production (1994–2018). Hard coal production at production levels becoming deeper every year does not change the technical parameters of extracting walls. No significant concentration of coal extraction was found, as the parameters of longwalls change regardless of the year, depth and amount of coal extracted changes.
During the last 4 years of the study, the average depth of coal production in the Pniówek mine rose from − 613 (2015) to − 665 m above sea level in 2018 (about 880 in 2015 to 930 m below ground level in 2018) which was 13 m deeper every year. Between 2015 and 2018, a greater amount of coal production was observed (JSW—internal reports).
Methane emissions
Budryk mine
The CMM from all the coal excavations of the Budryk mine was measured in the period from 1994 to 2018. From the beginning of the study to 2005, the total methane emission rose from 2.21 to 55.80 million m3/year (Fig. 8). In subsequent years (2006–2012) methane emission was around 40 million m3 of gas per year. From 2013 a large increase in methane emission was observed; in the last three years of the study (2016–2018), over 140 million m3 of CH4 was emitted yearly, which was three times more than the average emission in 1994–2012.
At the beginning, coal was mined at shallower, naturally degassed seams but when coal mining entered into a deeper zone with higher methane content, the total CH4 emission increased rapidly. The methane content and gas pressure increase with depth within the Main Trough area, including the Budryk mine, what is the main reason of the large increase in methane emission at greater depths in the mine. The related data, such as degassing, ventilation air methane (VAM), and specific methane emission, follow the trend of the total methane emission (Fig. 8). The Budryk mine started degassing of the coal seams in the fourth year after coal extraction had been started (in 1997) (Fig. 8). Before that time, all of the methane was released directly to air. It is worth mentioning that from 1997 to 2013 between 30 and 50% of all of the emitted methane was captured by the underground methane drainage system. When the total methane emission suddenly rose in the last 5 years of the research period, the share of degassing and utilising methane in internal mining processes also increased, to reach 70–88% in the period 2014–2018. The specific methane emission shows the real methane hazard that miners and mining authorities have to deal with. From the beginning of the research period to 1998 the specific methane emission was below 10 m3/Mg of extracted coal (Fig. 9). From 1999 until 2013 the amount of emitted gas was oscillating between 10 and 20 m3 of CH4 (Fig. 10). In the last five years of the study, the specific methane emission increased to 26 m3/Mg and was doubled (54–59 m3/Mg) in 2016–2018 (Fig. 9). The Budryk mine, as the youngest working coal mine in Poland, started coal extraction in 1994. In the geological past, shallow lying coal seams (up to about 500–600 m deep) were naturally degassed, owing to erosion and hydrodynamic changes in the rock mass in the northern part of the USCB before the Miocene period. The degassing process was facilitated by faults constituting migration pathways for methane. As a result, methane emission values correspond to the pattern A of the vertical methane distribution in the USCB. Shallower seams were emitting less than 40 million m3 of CH4 yearly during mining activities. As the depth of extraction increased, entering the primary methane maximum at the depth of 600 m (Fig. 4), the CH4 emission to mine excavations increased rapidly, exceeding 140 million m3 of gas in the last three years of the study (2016–2018). The increase in methane content in coal seams and surrounding rocks results in an increase in gas pressure in the rock mass (Figs. 5, 6a), which also affects the intensity of methane emission into mine workings.
Pniówek mine
The Pniówek coal mine has been producing coal much longer than Budryk; hence, all the data come from the period 1986–2018. When we take a look at the total methane emission and the related emission data, we will see that those trends are completely different than in the Budryk mine. The largest total CH4 emission values were observed in the late 1980s and at the early 1990s, when the coal was mining just below the sealed Miocene strata, where methane was accumulated in the coal seams as well as in porous rock strata in the geological past, forming the local methane maximum associated with the pattern B of the USCB vertical CH4 distribution (Sect. 4.1, Figs. 3, 4). The largest coal mine methane emission was reported in the period 1987–1989, when over 180 million m3 of gas was released to mine excavations over a one year period (Fig. 10). In subsequent years, the emission was decreasing from over 167 million m3 in 1990/91 to the average of 123 million m3 yearly during the next 26 years’ period (1992–2017). The VAM adopts a similar trend as the total CH4 emission, reaching maximum values from the beginning of the research to 1991, with the highest value in 1989, when over 109 million m3 of this dangerous gas was discharged out of the mine (Fig. 10). Over subsequent years, the VAM trend is stable with small rises and decreases, reaching the lowest value similar to that of the CMM in 2018, when only 60 million m3 of gas was removed by the ventilation systems out of the mine (Fig. 10).
Between 1991 and 2008, we can observe a decrease in specific methane emission with over 30 m3of methane emitted per one Mg of coal (Fig. 11). In 2008–2014, the CH4 emission over 40 m3/Mg was noticed with slight, but constant decrease in the following years until the end of the study period when the lowest emission was recorded: 25.51 m3 of CH4/Mg in 2018. In the period 2015–2018, coal production increased to over 3 million Mg/year and the total methane emission decreased to under 120 million m3/year (Fig. 10).
Due to complex and diversified faulting (Figs. 2, 3), geological structure and deeper coal extraction every year, the methane emission fluctuates in both mines with consistent trends. In the Budryk mine, the trend is increasing, but in the Pniówek mine, it is slightly, but constantly decreasing. Despite the different methane liberation trends, the total CH4 emission in both mines remains at the highest level in the Upper Silesian Coal Basin throughout the entire research period.
In addition to methane emissions in the Pniówek mine, much more dynamic events took place in the form of gas and rock outbursts. In 2002, during the blasting operations at the level of 1000 m, there was an outburst of approx. 250 m3 of grinded down coal and ejection of ~ 55,000 m3 of methane. The concentration of released methane in the mine air increased to ~ 86%.The gas and rock outburst in the neighbouring Zofiówka mine in 2005, which took 3 fatalities, resulted from the accumulation of methane in the mylonitic coal accompanying the two fault zones (Młynarczuk and Wierzbicki 2009; Jakubów et al. 2006; Kędzior 2012). The vertical distribution of methane content observed in the Pniówek mine is different from that in the Budryk mine. The difference concerns the occurrence of the zone secondarily saturated with methane under the Carboniferous top, which is evident by the high gas content in coal seams lying in this zone (Sect. 4.1.). The zone of increased pressure of free gas (7–8 MPa) associated with porous detritus lying at the uppermost part of the Carboniferous sediments is also important (see Sect. 4.1). Thus, coal extraction at the beginning of the study, when shallower seams were operated, was conducted under a higher methane hazard than when it was carried out in deeper seams in subsequent years. The secondary methane accumulation with methane content exceeding 10 m3/Mg coaldaf placed under the Miocene cover and also the occurrence of many faults (Fig. 3, see Sect. 4.1), considered as migration pathways for methane, were the cause of the high methane emission (over 160 million m3 CH4) to coal workings in a year period. In subsequent years, the total methane emission dropped to over 90 million m3 in 2018, which may be associated with a decrease in the methane content of the seams as the depth of extraction increased and as it entered the zone of reduced gas content and pressure. The deeper occurring primary gas-bearing zone has a lower methane content (< 10 m3/Mg coaldaf) than in the case of the secondary methane zone adjacent to the Miocene overburden (about 10 m3/Mg coaldaf) (Fig. 4).
To sum up, methane emissions in the studied mines are the result of natural factors (geological and gas content of the rock mass), influencing in the first place, and anthropogenic (mining) aspects acting additionally. Details are shown in the Table 4.
Environmental aspect
Methane was recognized as the second-most important and powerful anthropogenic greenhouse gas (GHG) with a global warming potential (GWP) ranging from 20 to 36 times greater than carbon dioxide over a 100-year time period and 86 times greater over a 20-year period (Archer 2011; IPCC et al. 2013; Etminam et al. 2016; US EPA 2019a). Coal mining production is one of the largest sources of the methane emission, estimated for 11% of CH4 emitted worldwide (US EPA 2019a, b; Global Methane Initiative 2020). Globally, the main methane emittants are: agriculture, wastes, biomass, coal mining, fuel combustion and natural emissions (Yusuf et al. 2012; Global Methane Initiative 2020). In Poland, the methane emitted to the atmosphere from underground coal mining accounts on 33.8% total methane emission in the country (Institute of Environmental Protection-National Research Institute 2020; Dreger 2021). When coal is mined, large amounts of CH4 are released from coal and surrounding strata to the mining atmosphere due to drilling, grounding, transportation, explosives, etc. (e.g. Karacan et al. 2011; Kędzior and Dreger 2019). Methane emitted to the atmosphere is a mixture of unused captured gas (from underground drainage) and methane coming from the ventilation air emission (Tutak and Brodny 2019; Dreger 2021). Methane emission from mining ventilation shafts contributes the most to global methane emission from mining industry, nevertheless CH4 is a potent source of energy and can be collected by underground drainage and can be used economically in the future (Global Methane Initiative 2020; Swolkień 2020; Dreger 2021). Unfortunately, in the Upper Silesia Coal Basin only 25% of all emitted methane is captured by underground drainage system. The vast majority of released gas to the coal workings is disposed by VAM (75%) (Tutak and Brodny 2019; Dreger 2021; Szlązak and Swolkień 2021). Unluckily, it is impossible to capture all of the emitted gas and gas mixture in the areas affected by mining works. The greenhouse effect magnification from coal mines does not stop, even when the mine is closed. The methane liberation from non-extracted coal seams, overlying and underlying seams can be active up to 15 years after colliery closuring. This problem was the purpose of numerous studies (e.g. Pokryszka and Tauziede 2000; Franklin et al. 2004; Krause and Pokryszka 2013; Kholod et al. 2020).
Besides the great heat absorption, methane is harmful to the human health and crops. There were recognized many indirect effects of CH4 emission like heart and lungs diseases and yield losses (West and Fiore 2005; UNEP Synthesis Report 2011).
In 2018, over 1.9 million Mg of methane was emitted in the territory of Poland, including 0.53 million Mg from the USCB coal mines. It is worth to mention that 20% of all emitted GHG in Poland is covered by CH4 but Polish gassy mines are responsible for only 3% GHG in the country (Dreger 2021). Coal production industry in Poland and worldwide will be struggling with more complex geological and mining conditions and also, with greater depths of mining when more methane is going to be emitted (Kędzior and Dreger 2019; Tutak and Brodny 2019; Karacan et al. 2021). The development of VAM gas production is the key solution to limit the CH4 emission to the atmosphere. However, in Poland, to ensure safety, the concentration of methane in the VAM has to be reduced to ≤ 0.75% in the ventilation shafts. Thus, the energy production from low caloric fuel is ineffective (e.g. Honysz 2015; Szlązak and Swolkień 2021). Globally, several technologies were developed to use air mixture with low CH4 concentration in the turbine engines. The list of technologies can be found at: CMM energy (2021), EPA (2019a, b), Szlązak and Swolkień (2021).
Conclusion
The Budryk and Pniówek mines belong to the most gassy mines in the Upper Silesian Coal Basin. However, both are located in different parts of the basin, which are characterised by both different geological structure and spatial distribution of gas content. At the Budryk mine, the youngest in the basin, coal mining was initially carried out (1990s) in a shallow naturally degassed zone, then it entered into a deeper zone with high methane content of 12 and more m3/Mg coaldaf. This resulted in a sharp increase in methane emissions from around 2 to over 140 million m3 of methane per year (late 2010s).
At the Pniówek mine, coal was initially mined in high-methane seams occurring in the secondary methane-bearing zone with high methane content in coal seams (> 10 m3/Mg coaldaf) and elevated free gas pressure (7–8 MPa) in weathered rocks, located just below the sealing Miocene overburden. This resulted in record-high methane emissions in the initial extraction period (1980s), reaching 180 million m3 annually. In subsequent years, methane emissions decreased to around 100 million m3 in 2018 with numerous fluctuations throughout the entire research period. This can be explained by the lower methane content and gas pressure in coal seams at a greater depths associated with the occurrence of a reduced methane content zone and the primary gas-bearing zone occurring deeper, but with a lower gas content than the shallow, secondary one. Thus, it may seem that the vertical zonation of the gas content in seams is the main factor that controls methane emissions in the analysed mines, because the temporal variability of methane emissions coincides with the depth of coal extraction corresponding to individual gas zones.
Faults, breaks and rock discontinuities are an important factor of methane migration, because in their vicinity a decrease or increase in gas content and gas pressure has been observed. Often, methane had migrated through faults in the geological past, and thus fault zones can also be now a source of methane emissions into mine workings. In special circumstances, they can also cause more dynamic phenomena, such as gas and rock outbursts, which took place in the Pniówek and Zofiówka mines.
Also important are the mining factors affecting methane emissions, such as the intensity of coal mining, the size of the mining longwalls, their number and the presence of goafs, which are an important source of methane emissions. Along with significant methane emissions in both mines, methane is captured by methane removal stations, which has a positive impact on safety of miners at work, economic balance of the mines and environmental protection (reduction of greenhouse methane emissions to the atmosphere).
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Acknowledgements
This study was undertaken in the framework of the activities of the University of Silesia in Katowice and was funded by the University of Silesia, Institute of Earth Sciences (WNP/INOZ/2020_ZB32). The authors are grateful to the employees of Budryk mine, especially to Mr. Dariusz Kluczniok, Adam Kurpas, Jacek Kurpan and from Pniówek mine to Mr. Zenon Fojcik and Paweł Faryniarz and also to the employees of the CLP-B Sp. z o.o. in Jastrzębie-Zdrój and for their kind cooperation and leads during data collection for this research.
Funding
This study was undertaken in the framework of the activities of the University of Silesia in Katowice and was funded by the University of Silesia, Institute of Earth Sciences (WNP/INOZ/2020_ZB32).
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Dreger, M., Kędzior, S. Methane emissions against the background of natural and mining conditions in the Budryk and Pniówek mines in the Upper Silesian Coal Basin (Poland). Environ Earth Sci 80, 746 (2021). https://doi.org/10.1007/s12665-021-10063-4
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DOI: https://doi.org/10.1007/s12665-021-10063-4