Abstract
27Al, 51V, 52Cr, 55Mn, 56Fe and 58Ni nuclei are some structural fusion substances. The neutron incident energy around 14–15 MeV is adequate to excite the nucleus for the reactions such as (n, p), (n, d), (n, 2n), (n, t), and (n, α). For fusion reactor technology, the reaction cross-sectional data have a critical importance in fusion reactors and development. Neutron irradiation produces considerable modifications in the mechanical and physical properties of each of the structural fusion material systems raising feasibility questions and design limitations. In this paper, for some structural fusion materials (n, α) reactions such as 52Cr(n, α)49Ti, 51V(n, α)48Si, 27Al(n, α)24Na, 58Ni(n, α)55Fe, 56Fe(n, α)53Cr and 55Mn(n, α)52V were done up to 40 MeV incident neutron energy. In the calculations, the equilibrium and pre-equilibrium impacts have been used. Calculations have been carried out with TALYS 1.9 and EMPIRE 3.2 (Malta) nuclear model codes. Results from performed calculations have been compared with the experimental nuclear reaction data, ENDF/B-VII.b4, JENDL-4.0 and JEFF-3.2 evaluated data.
Similar content being viewed by others
Avoid common mistakes on your manuscript.
1 Introduction
Nuclear fusion, sometimes referred to as thermonuclear fusion, is a process where two light atomic nuclei come together to form a heavier nucleus [1]. Nuclear fusion can be one of the most attractive sources of energy from the viewpoint of safety and minimal environmental impact. The development of fusion materials for the safety of fusion power systems and understanding nuclear properties is important. The success of fusion power system is dependent on the performance of the first wall, blanket or divertor systems. So, the performance of structural materials for fusion power systems, understanding nuclear properties systematic and working out of (n, α) reaction cross sections are very important. Neutron scattering cross sections and neutron emission differential data have a critical importance on fusion reactors. In fusion reactor structures, a serious damage mechanism has been gas production in the metallic resulting from diverse nuclear (n, p) and (n, a) reactions above a certain threshold energy. [2,3,4,5,6,7,8,9,10] The experimental cross sections are available in EXFOR for neutron-induced reactions. These data can be extensively used for the investigation of the structural materials of the fusion reactors, radiation damage of metals and alloys, tritium breeding ratio, neutron multiplication and nuclear heating in the components, neutron spectrum, and reaction rate in the blanket and neutron dosimetry.
Nuclear data are required to explain reaction mechanisms and to develop more nuclear models. Also neutron cross sections around 14 MeV are important from the viewpoint of fusion reactor technology, especially for the calculation of nuclear transmutation rates, nuclear heating and radiation damage to the materials used in the construction of the core and inner walls of the reactor.
In the present work, neutron incident reaction cross sections for some structural fusion materials such as 27Al(n, α)24Na, 51V(n, α)48Sc, 52Cr (n, α) 49Ti, 55Mn(n, α)52V, 56Fe (n, α) 53Cr, and 58Ni(n, α)55Fe have been calculated up to 40 MeV by using the equilibrium and pre-equilibrium models. Calculations have been carried out with TALYS 1.9 and EMPIRE 3.2 (Malta) nuclear model codes. Results from performed calculations have been compared with the experimental nuclear reaction data, ENDF/B-VII.b4, JENDL-4.0 and JEFF-3.2 evaluated data.
2 Theoretical calculations methods of nuclear reaction cross sections
The elementary pre-equilibrium differential cross section for the emission of a particle k with emission energy EK can then be expressed in terms of s, the composite-nucleus formation cross section \( \sigma \)CF, and an emission rate Wk [11,12,13,14,15,16,17,18,19,20]:
where the factor P represents the part of the pre-equilibrium population that has survived emission from the previous states and now passes through the (p \( \pi \), h\( \pi \), p \( \upsilon \), h\( \upsilon \)) configurations, averaged over time. \( p_{\pi }^{0} = Z_{p} \) and \( p_{\upsilon }^{0} = N_{p} \) are the initial proton and neutron particle numbers, respectively, with Zp (Np) the proton (neutron) number of the projectile. \( h_{p}^{0} = h_{\upsilon }^{0} = 0 \) and \( h_{v} = p_{v} - p_{v}^{0} \), for any exciton state in the reaction process; so that the initial hole numbers are \( h_{p}^{0} = h_{v}^{0} = 0 \) for primary pre-equilibrium emission. Particle emission only occurs from n = 3 (2p1 h) and higher exciton states [21,22,23,24,25,26,27,28,29,30,31,32,33,34,35].
For calculating the excitation functions, we used two different nuclear reaction program codes. “Exciton” and “two-component exciton” models were used in TALYS 1.9, EMPIRE 3.2 (Malta) nuclear reaction program code for pre-equilibrium reaction systematics, respectively [12, 13].
In the two-component exciton model, which is the default model for TALYS reaction cross-sectional computations, the holes and particles are followed throughout the reaction. The notation for the following equation gives the numbers of particles which could be proton or neutron and holes as pπ(pν) and hπ(hν), respectively. From this, the proton exciton number is defined as \( n_{\pi } = p_{\pi } + h_{\pi } \) and the neutron exciton number as \( n_{\upsilon } = p_{\upsilon } + h_{\upsilon } \) which give us to construct the charge-independent particle number as \( p = p_{\pi } + p_{\upsilon } \), the exciton number as \( n = n_{\pi } + n_{\upsilon } \) and the hole number as \( h = h_{\pi } + h_{\upsilon } \).
EMPIRE uses the Exciton [14] model PCROSS module for the reaction in cross-sectional computations of pre-equilibrium reactions. A unified model is used by the exciton model that is the solution of a key equation that was previously represented by Cline [15] and Ribansky [16].
3 Results and discussions
In the present work, for some structural fusion materials (n, α) reactions such as 27Al(n, α)24Na, 51V(n, α)48Sc, 52Cr (n, α)49Ti, 55Mn(n, α)52V, 56Fe (n, α)53Cr, and 58Ni(n, α)55Fe have been calculated up to 40 MeV incident neutron energy. Results from performed calculations have been compared with the experimental nuclear reaction data, ENDF/B-VII.b4, JENDL-4.0 and JEFF-3.2 evaluated data. A reasonable agreement with theoretical excitation functions and experimental was obtained. It can be said that at least this work helps to show the way to the later experimental studies and contributes to the new studies on (n, α) reaction cross sections . The results can be concluded and summarized as follows:
3.1 Excitation function of 27Al(n, α)24Na reaction
Figure 1 shows the calculated excitation functions for the nuclear reactions 27Al(n, α)24Na in comparison with the experimental nuclear reaction data, ENDF/B-VII.b4, JENDL-4.0 and JEFF-3.2 evaluated data. The experimental cross-sectional datasets are between 3.5 and 40 MeV, and the data around 9 \( E \) 17 MeV show big discrepancies. The TALYS 1.9 follows the trend of the experimental nuclear reaction data. The pre-equilibrium spectra calculations of emitted (\( \alpha \)) for 27Al nuclei are in reasonable agreement with experimental nuclear reaction data and with ENDF/B-VIII.b4, JEFF-3.2 and JENDL-4.0 files (evaluations international libraries). Generally, there is a good agreement between the cross sections calculated with TALYS 1.9 and the experimental nuclear reaction data. The results of EMPIRE 3.2 (Malta) give unacceptable results between 0 and 13 MeV and strongly underestimate between 15 and 26 MeV. The estimation of EMPIRE 3.2 (Malta) is acceptable between 28 and 38 MeV.
3.2 Excitation function of 51V(n, α)48Sc reaction
Figure 2 shows the calculated excitation curve for the nuclear reactions 51V(n, α)48Sc in comparison with the experimental nuclear reaction data, ENDF/B-VII.b4, JENDL-4.0 and JEFF-3.2 evaluated data. The experimental cross-sectional datasets are between 2.96 and 38.5 MeV. The theoretical investigation using TALYS 1.9 & EMPIRE 3.2(Malta) indicates the emitted alpha spectra, and the compound contribution is dominant by the pre-equilibrium contribution which mainly comes from the high-energy emitting alphas and the low-energy emitting alphas. The theoretical investigation using TALYS 1.9 & EMPIRE 3.2(Malta) follows the trend of the experimental nuclear reaction data, but EMPIRE 3.2(Malta) strongly overestimates above 11 MeV, while TALYS 1.9 overestimates over 16 MeV. The equilibrium calculations of the TALYS 1.9 and EMPIRE 3.2(Malta) are mostly in good agreement with the experimental nuclear reaction data and with ENDF/B-VIII.b4 and JENDL-4.0.files (evaluations international libraries).
3.3 Excitation function of 52Cr (n, α)49Ti reaction
Figure 3 shows the calculated excitation curve for the nuclear reactions 52Cr (n, α)49Ti in comparison with the experimental nuclear reaction data, ENDF/B-VII.b4, JENDL-4.0 and JEFF-3.2 evaluated data. The experimental nuclear reaction data are rather few for 52Cr (n, α)49Ti reactions. When there are more experimental values for these reactions, more reliable results can be obtained. The evaluated nuclear data files ENDF/B-VIII.b4, JEFF-3.2 and JENDL-4.0 show significant discrepancies in energy between 0 and 40 MeV. The results of the theoretical nuclear reaction model calculations follow the trend of the experimental values, but the estimation of TALYS 1.9 is much better.
3.4 Excitation function of 55Mn(n, α)52V reaction
Figure 4 presents the excitation curve of 55Mn(n, α)52V nuclear reaction. The experimental nuclear reaction data are between 2.96 and 19 MeV, and the data around 12 \( E \) 19 MeV show very large discrepancies. The equilibrium results based on the Hauser–Feshbach formalism give lower results than experimental cross-sectional data. The pre-equilibrium calculations with exciton model give the lowest outcomes. The pre-equilibrium spectra calculations using TALYS 1.9 are mostly in good agreement between 13 and 15 MeV with experimental cross-sectional data, while EMPIRE 3.2 (Malta) overestimates between 13 and 20 MeV. The results of the theoretical nuclear reaction model calculations follow the trend of the experimental cross-sectional data, but the estimation of TALYS 1.9 is much better.
3.5 Excitation function of 56Fe (n, α)53Cr reaction
Figure 5 presents the excitation curve of 56Fe (n, α)53Cr nuclear reaction. The experimental nuclear reaction data are rather few for 56Fe (n, α)53Cr reactions. When there are more experimental values for these reactions, more reliable results can be obtained. The results of the theoretical nuclear reaction model calculations follow the trend of the experimental cross-sectional data, but the estimation of TALYS 1.9 is much better.
3.6 Excitation function of 58Ni(n, α)55Fe reaction
Figure 6 presents the excitation curve of 58Ni(n, α)55Fe nuclear reaction. The experimental nuclear reaction data are rather few for 56Fe (n, α)53Cr reactions. When there are more experimental cross-sectional data for these reactions, more reliable results can be obtained. The excitation functions obtained using TALYS 1.9 & EMPIRE 3.2 (Malta) exhibit very similar trends with each other, but the estimation of TALYS 1.9 is much better. The evaluated nuclear data files ENDF/B-VIII.b4 and JENDL-4.0 show significant discrepancies in energy between 0 and 40 MeV.
4 Conclusions
In the present work, for some structural fusion materials (n, α) reactions such as 27Al(n, α)24Na, 51V(n, α)48Sc, 52Cr (n, α)49Ti, 55Mn(n, α)52V, 56Fe (n, α)53Cr, and 58Ni(n, α)55Fe have been calculated. Results from performed calculations have been compared with the experimental nuclear reaction data, ENDF/B-VII.b4, JENDL-4.0 and JEFF-3.2 evaluated data. The calculation results have been compared with the available experimental data, and the conclusions can be drawn as follows:
-
1.
In general, the alpha emission spectrum of neutron bombardment of 27Al, 51V, 52Cr, 55Mn, 56Fe, and 58Ni is in agreement with the experimental data for the TALYS 1.9 models and EMPIRE 3.2 (Malta) Exciton model results.
-
2.
The results of the theoretical nuclear reaction model calculations follow the trend of the experimental points, but the calculation of TALYS 1.9 is much better.
-
3.
More theoretical and experimental works are needed, as a result, because the measurements of the investigated (n, α) reaction cross sections in the literature are not very large.
-
4.
In the present study, the different nuclear reaction program codes used show rather important differences both in shape and in size.
References
P Relly, R Aversa, K Samuel, A. Antonio and F. Ion Tiberiu Petrescu Am J Eng Appl Sci. 10 703–708 (2017)
M Yiğit Appl Radiat Isot. 105 15 (2015)
M Yiğit, E Tel J Fusion Energy 35 585 (2016)
T Siddik J Adv Phys 6 18–25 (2017)
T Siddik EPJ Web Conf 128, 01002 (2016)
T Siddik J Fusion Energy 34 2015
T Siddik J Fusion Energy 32 (2013)
T Siddik Balkan Phy Lett 22, 221012 104–118 (2013)
E Tel, S Akça, A Kara, M Yiğit, A Aydın, J Fusion Energy 32 531–535 (2013)
H Azizakram, M Sadeghi, P Ashtari, F Zolfagharpour Appl Radiat Isotopes 112 147–155 (2016)
M Yiğit, E Tel, A Kara J Fusion Energy 32 362–370 (2013)
S Koning, S Hilaire Goriely Talys-1.9 User’s Manual (2017)
M Herman, R Capote, M Sin B V Trkov, P Carlson, y Oblozinsky, C M Mattoon, H Wienkey, S Hoblit, Young-Sik Cho, G P A Nobre, V Plujko, V Zerkin Empire-3.2 Malta User’s Manual, Brookhaven National Lab (2013)
J J Griffin Phys Rev Lett 17 478 (1996)
C K Cline Nucl Phys A 193 417–437 (1972)
I Ribansky, P Oblozinsky, E Betak, Nulear Phys A 205 545–560 (1973)
H L Pai, D G Andrews Can J Phys 56 944–949 (1978)
J Joseph Jeremiah, D Suchiang, B M Jyrwa Ann Nuc Energy 43 208 (2012)
E E Bloom J Nucl Mater 258–263 7–17 (1998)
M Yiğit, E Tel Nuc Sci Techn. 28 165 (2017)
H Şahan, E Tel, M Yiğit J Fus Energy 34 16–23 (2015)
E.Tel, M.Yiğit, G.Tanır, J Fusion Energy 31 184–190 (2012)
P. Obložinský Evaluated Nuclear Data, Handbook of Nuclear Engineering (2010)
M B Chadwick, P Oblozinsky, M Herman, N M Greene, R D McKnight, D L Smith, P G Young, R E MacFarlane, G M Hale, R C Haight, S Frankle, A C Kahler, T Kawano, R C Little, D G Madland, P Moller, R Mosteller, P Page, P Talou, H Trellue, M White, W B Wilson, R Arcilla, C L Dunford, S F Mughabghab, B Pritychenko, D Rochman, A A Sonzogni, C Lubitz, T H Trumbull, J Weinman, D Brown, D E Cullen, D Heinrichs, D McNabb, H Derrien, M Dunn, N M Larson, L C Leal, A D Carlson, R C Block, B Briggs, E Cheng, H Huria, K Kozier, A Courcelle, V Pronyaev, S C van der Marck, ENDF/B-VII.0, Nucl Data Sheets. (2006)
D Fiscaletti,A Sorli, Found Sci (2015) 20 387–398 (2014)
B Pandey, Anna Nuclear Energy 38 731–920 (2011)
M Yiğit Appl Radiat Isotopes 139 151–158 (2018)
L Junhua, L An, L Jiang, L He, Appl Radiat Isotopes 98 40–43 (2015)
M Yiğit Nuclear Eng Technol, 50 411–415 (2018)
L Junhua, Z Feng, L An, L Jiang, L He Radiat Phys Chem (2016)
M Yiğit, A. Kara, J Radioanal Nucl Chem 314, Issue 3, pp 2383–2392 (2017).
M Yiğit, E Tel, İ H Sarpün, Nucl Instr Methods Phys Res Sect B Beam Interact Mater Atoms 385 1–94 (2016)
V K Mulikz H Naik, S V Suryanarayana, S D.Dhole, P M Prajapati, B S Shivashankar, K C Jagadeesan, S V Thakre, V N Bhoraskar, A Goswami J Radioanal Nucl Chem 296 1321–1329 (2013)
M Yiğit, E Tel, G Tanır J Fusion Energy 32 336–343 (2013)
M B Chadwick M Herman b P Obložinsky M E DunncY Danond A C KahleraD L Smithe B Pritychenkob G Arbanasc R Arcillab R Brewera D A BrownbfR Capoteg A D Carlsonh Y S Chom H Derrienc K Guberc G M Halea P G Younga, Nuclear Data Sheets (2011)
Experimental nuclear reaction data (EXFOR), Database version of 2017.04.03, http://www-nds.iaea.org/exfor/exfor.htm
Author information
Authors and Affiliations
Corresponding author
Rights and permissions
About this article
Cite this article
Siddik, T. Theoretical cross-sectional calculation of some structural fusion material on (n, α)-induced reactions. Indian J Phys 93, 921–925 (2019). https://doi.org/10.1007/s12648-018-1349-3
Received:
Accepted:
Published:
Issue Date:
DOI: https://doi.org/10.1007/s12648-018-1349-3
Keywords
- (n, α) cross section
- Nuclear reactions
- TALYS 1.9 nuclear model code
- EMPIRE 3.2 (Malta) nuclear model code