Introduction

Aeolian (wind) soil erosion is a common process in arid regions that can lead to dust emission into the atmosphere. Dust emission has significant impacts on the Earth’s systems depending on the physical and chemical characteristics of the topsoil (Shao, 2008). The emission of dust from soils is a major concern due to soil degradation by loss of clays (< 2 μm) and fine silt (< 10 μm), and absorbed nutrients. In addition, emission of PM10 and PM2.5 (particulate matter that is smaller than 10 and 2.5 μm in diameter, respectively) to the atmosphere increases air pollution and health risks particularly in arid environments (Ganor et al., 2009; Krasnov et al., 2014; Vodonos et al., 2014; Yitshak-Sade et al., 2015).

The surface characteristics determine the critical value (threshold) of wind (friction) velocity at which the aerodynamic drag is enough to dislodge particles from the surface and initiate their transport (Bagnold, 1941; Kok et al., 2012). Direct aerodynamic lifting is a dominant mechanism for loose fine-particle emission such as PM10. However, emission of cohesive fine particles (e.g., clays) is enabled only under higher wind velocities and/or under saltation flow (Bagnold, 1941; Kok et al., 2012). The presence of sand particles in the soil enables the entrainment of fine particles (clay and silt) by ballistic impact (saltation bombardment) (Shao et al., 1993). Surface cover such as vegetation and rock fragments increases surface roughness and thus reduces near-surface wind velocities and erosion (Wolfe and Nickling, 1993; Gillies et al., 2006; Li et al., 2005). Crusted surface layer significantly reduces soil erodibility, where the strength of crusts varies with the composition and distribution of the binding media (Belnap and Gillette, 1998; Langston and McKenna Neuman 2005; Zaady et al., 2014). Among the soil properties, the dry aggregate size distribution of the topsoil is a major factor influencing the resistance to wind erosion. High proportion of erodible fraction (EF) (aggregates >840 μm) in the upper layer of the soil surface increase its erodibility (Hevia et al., 2007; Van Pelt et al., 2013; Li et al., 2015; Swet and Katra, 2016).

Desert environments are associated with a diverse range of geomorphological landforms such as desert pavements, playas, and alluvial fans that constitute source areas of dust emission (Bacon et al., 2011; Sweeney et al., 2011; Al-Dousari and Al-Awadhi 2012). The specific surface properties and the presence of different features on the surface (e.g., vegetation, crusts or rock fragments) control the magnitude of dust-related PM10 emission from a specific soil (King and Nickling, 2005; Bacon et al., 2011; Hoffmann and Funk, 2015). It has been shown that topsoil disturbance can significantly accelerate aeolian erosion and PM10 flux compared with natural (non-disturbed) crusted topsoil’s (Sharratt et al., 2010; Baddock et al., 2011; Singh et al., 2012).

Soils in many deserts throughout the world are subjected to strain of increased human pressure and thus changes in their physico-chemical properties and potential of dust emission. The underlying assumptions about the surface complexity in a dust source incorporated into the dust emission models limit their accuracy. Knowledge about the variability of actual dust emission at various scales is still lacking. Katra and Lancaster (2008) demonstrated spatio-temporal variability in the surface sediments of identified source area to reveal the potential changes for dust emissions over time. The study aim was to examine variations in PM10 fluxes due to surface composition and topsoil disturbance. Aeolian field experiments by a boundary layer wind tunnel were applied to quantify the PM10 fluxes from a study area with typical soil characteristics of arid dust sources.

Material and methods

Experimental plots

The study was conducted on desert soils of the Negev (Yamin Plain), Israel. The tested soils in Yamin Plain have not been exposed to anthropogenic activities as it is a part of natural reserves. The annual average rainfall is ~75 mm. The silt-loam soils are characterized by low content of organic matter (< 1 %) and a wide range of sand/clay percentage depending on the specific site location. During the majority of the year, the topsoil is dry and is subjected to intensive aeolian erosion. The dominant wind direction is northwest during the day and alternates to southwestern along the night. The wind velocities can exceed up to 13 m s−1 (measured 6 m above the soil surface).

Experimental plots were designed within a closed area without human interference during the last six decades. The experimental plots for the soil sampling and the aeolian experiments (see below) were representative of the surface cover in the area (Fig. 1): an extensive coverage of mechanical crust (MC), sparse vegetation-shrubs cover (SV) with a typical distance of about 2 m between adjunct shrubs, and soil mechanical crust covered with different sizes (up to 15 cm in diameter) of rock fragments (RF).

Fig. 1
figure 1

Location of the experimental plots (Yamin Plain) in the Negev, Israel, with the surface characteristics of sparse vegetation cover (SV), rock fragments (RF), and mechanical crust (MC)

Soil analysis

In each experimental plot (SV, RF, MC), dry soil samples were taken from the topsoil (0–2 cm), which is the exposed layer to wind erosion processes. A total of 48 samples (n = 16; for each SV, RF, and MC soil type) were analyzed in the lab for soil properties using soil science methods (Klute, 1986; Rowell, 1994; Pansu and Gautheyrou, 2006) as follows.

Aggregate size distribution (ASD) was conducted by using the dry sieving method. The samples were placed on a set of six sieves in the diameters of 63–4000 μm and were shaken in moderate amplitude for 8 min by an electronic sieving apparatus (RETSCH AS 300 Control). After sifting, every size fraction was weighted separately. In the fraction of >2000 μm, rock fragments were extracted from the rest of the soil particles. The results have been used to calculate the mean weight diameter (MWD) of the soil aggregates.

Particle size distribution (PSD) was performed by ANALYSETTE 22 MicroTec Plus laser diffractometer (www.fritsch.com), which measures particles in the size range of 0.08–2000 μm. The preparation of each sample includes splitting for replicate samples by a micro-splitter device and the removal of distinct organic matter. For the analysis, the replicates (100 mg) of each sample were dispersed in a Na-hexametaphosphate solution (0.5 %) and by sonication (38 kHz). PSD data was calculated using the Fraunhofer diffraction model. By using MasControl software, relevant parameters were determined statistically: mean size, median, and modes in multiple modal distributions, sorting values, size fraction weights. The size resolution for analyses was 1 μm. The results allow the determination of the soil texture of sand (50–2000 μm), silt (2–50 μm), and clay (< 2 μm) according to the USDA classification.

Aeolian experiments

Aeolian experiments in the field were conducted in dry soils (Fig. 1) with a boundary-layer wind tunnel. Boundary-layer wind tunnels enable aeolian simulations under standardized quasi-natural wind conditions (Shao, 2008) and provide quantitative information on aeolian particle transport, including sand fluxes (Katra et al., 2014) and dust emission rates from soils (Tanner et al., 2016). The wind tunnel used in this study has a cross sectional area in the order of 0.5 × 0.5 m with open-floored working sections of up to 10 m length (see more details in Swet and Katra, 2016). The airflow in the tunnel is generated by an axial fan up to a maximum velocity of 18 m s−1. Instruments installed in the test section of the tunnel enable quantification of wind characteristics and sediment transport.

The aeolian experiments in each plot were performed under two topsoil conditions: (1) natural surfaces (a non-disturbed topsoil) and (2) disturbed surface in which the topsoil was artificially disturbed at the upper 2 cm layer by the same mechanical operation in all plots to simulate disaggregation of the topsoil. In each experimental plot, 12 sub-plots (replicas) were defined in size area of 0.5 m × 10 m in accordance with the dimensions of the experimental system. A total of 72 experiments were conducted in the field (3 plots, 2 soil treatments, 2 wind speeds, and 6 replicas).

The tunnel fan was set in two frequencies; the first of 32 Hz represents medium wind speed in the study area and above the threshold of particle transport (~5 m s−1), and the second of 44 Hz represents higher wind speed of typical aeolian erosion conditions in the studied area (~ 9 m s−1). In each experimental plot, the mean wind velocity profile was measured under both fan frequencies (32 and 44 Hz). The shear velocities (u *) calculated by the semi-empirical logarithmic law of Karman (Bagnold, 1941) were at the range of 0.31–0.69 m s−1, depending on the fan frequency and the surface composition (plot). During each test, the PM10 concentrations in the wind tunnel were measured by a particulate monitor (HAZ-DUST EPAM-5000, www.skcinc.com). The EPAM-5000 uses light scattering technique to measure particle concentration and provide real-time data recordings at the range of 0.01 to 200 mg m−3 (accuracy ±10 % to filter gravimetric test dust). The recorded PM10 data over time were converted into fluxes from the soil surface based on the wind tunnel dimensions and area of the experimental plot (3.75 m2). The sand transport during the experiment was measured by a cylindrical piezo-electric sensor (www.sensit.com) that converts the impact energy of the saltating particles into electrical impulses. The Sensit data were logged as number of impact-particles (NP) on a Campbell Scientific Inc. CR-1000X data logger at 1 s intervals. The NP values were converted into horizontal saltator flux (mg m−2 s−1) considering the sensor impact area and the weight of the sand particles in the studied area at the size of 100–200 μm (the mean weight of 1 particle =57 μg). Each experiment lasted 400 s, representing a typical trend of soil erosion under limited sediment supply (Tanner et al., 2016).

Results and discussion

Topsoil characteristics

The PSD results show a tri-modal distribution in all the experimental plots (Fig. 2). The results represent both conditions of natural surface and disturbed surfaces – the samples were extracted prior to aeolian experiments in each condition, considering that no changes in PSD are expected in response to a short-term disturbance of the topsoil. SV soil was coarser, with significantly higher sand content than RF and MC soils. RF soil showed higher amount of clay compared to SV and MC soils. Differences in PM10 content in the soil were noted between the plots, in which the highest content was in MC plot while the lowest content in SV.

Fig. 2
figure 2

Average particle size distribution (PSD) by the laser diffractometer technique in the topsoils of sparse vegetation (SV), rock fragment (RF), and mechanical crust (MC). The size fractions derived from the PSD is presented in the box

Aggregate size distribution was measured for each plot and soil conditions (natural and disturbed) (Fig. 3). In both soil conditions, the amount of aggregate at the size fraction of 250–500 μm was higher compared with the other size fractions. The disturbance of the topsoil led to elimination of aggregates >2000 μm and to a reduction in the content of aggregates in the size fraction of 1000–2000 μm. Accordingly, the amounts of the smaller size fractions 500–1000, 250–500, 125–250, 63–125, and <63 μm were increased following disturbance by 18, 26, 34, 34, and 63 %, respectively. The most significant change occurred in MC plot with increased amount of the erodible fraction (< 500 μm) following disturbance.

Fig. 3
figure 3

Aggregate size distribution (ASD) of SV, RF, and MC in natural (a) and disturbed (b) surface conditions

MWD driven from ASD was calculated for both conditions of natural and disturbed surfaces. The relatively low MWD values in natural condition in all plots (362.5, 512.5, and 433 μm in SV, RF, and MC, respectively) indicate a potential of high susceptibility to wind erosion due to high proportion of erodible aggregate size fractions. The MWD values were lower at all experimental plots following disturbance of the natural surfaces (314.1, 283.2, and 253.3 μm in SV, RF, and MC, respectively).

Variations in PM10 flux

The in situ aeolian experiments enabled the measurement of PM10 emission from the topsoil following wind erosion. A similar trend in PM10 emission was observed for natural and disturbed surfaces in both lower (32 Hz) and higher (44 Hz) wind velocities at all experimental plots (Fig. 4). The dust emission is characterized by increased PM10 concentrations in the first few seconds of the run up to a peak value, a relatively moderate decline followed by a steady-state phase which consist low PM10 concentrations. In all cases, increased wind velocity resulted in higher PM10 concentration over time (Fig. 3). At lower velocity (32 Hz frequency), the disturbance of the topsoil did not lead to a significant increase in PM10 concentrations at all plots. At high wind velocity (44 Hz frequency), significantly higher PM10 concentrations were recorded in all experiments. These changes particularly in the natural topsoil are indicative of the importance of wind velocity.

Fig. 4
figure 4

PM10 concentrations measured during the aeolian experiments in SV, RF, and MC plots at 32 and 44 Hz frequencies and in natural and disturbed surface conditions

In order to estimate PM10 losses from the topsoils, the PM10 concentrations measured during the aeolian experiments were converted into PM10 fluxes from the soil (mg m−2 min−1) (Table 1). In all topsoil conditions and wind velocities, MC plot showed the highest PM10 flux (except for the disturbed topsoil in frequency of 44 Hz) although with no statistical significance (p ≤ 0.05). Significant differences between the plots were noted only at disturbed topsoil in a 44 Hz frequency, were PM10 flux from SV plot was significantly higher than RF plot. In both SV and MC plots, significantly higher PM10 flux was obtained under 44 Hz in disturbed soil condition. RF plot showed no significant differences between the different topsoil conditions and wind velocities.

Table 1 Average PM10 flux from topsoil at SV, RF and MC in different fan frequencies and different topsoil conditions

The PM10 fluxes at the lower velocity (32 Hz frequency) were increased by 144.2 % in SV plot due to topsoil disturbance (Table 1). At the higher wind velocity (44 Hz frequency), the PM10 fluxes were increased by 98.5–336.8 % in all plots. The results indicate that the effect of topsoil disturbance on PM10 fluxes is stronger under higher wind velocities as demonstrated also by Li et al. (2015). However, the increase in wind velocity from 32 to 44 Hz in the natural topsoils led to increase in PM10 fluxes of 261.6 % (MC), 316.6 %, and 1164.2 % (SV). These changes are indicative of the importance of wind velocity in dust emission rates in the studied area. A positive linear correlation (R 2 = 0.73) was found in the current study between the wind shear velocities (u*) and the PM10 fluxes in the natural topsoils of all the plots. The correlation supports the findings of previous work (e.g., Sweeney and Mason, 2013).

Impact of saltators

Dust particle is emitted from soils through physical mechanisms, including direct aerodynamic lifting, saltation bombardment and disaggregation/self-breakdown of saltating (sand-size) aggregates (Shao, 2008; Kok et al., 2012; Swet and Katra, 2016). The relationships between the soil saltators (i.e., sand particles and/or sand-sized aggregates) and PM10 fluxes from the topsoil were examined. The results indicate an exponential correlation between the saltators and PM10 emission in all soil compositions (Fig. 5). The strongest correlation was obtained in RF (R 2 = 0.84) followed by SV (R 2 = 0.78) and MC (R 2 = 0.52). The higher content of soil PM10 in MC plot compare to the other plots (Fig. 2) may contributed more to the total PM10 fluxes via direct aerodynamic lifting mechanism rather than saltation bombardment and disaggregation, which can explain the weaker correlation to saltator flux obtained in this plot. In contrast, the significantly higher amount of sand particles in SV plot (Fig. 2) can be associated with the highest PM10 fluxes measured at the disturbed topsoil at 44 Hz (Table 1) through the saltation bombardment mechanism.

Fig. 5
figure 5

Dependence of PM10 flux on saltators flux recorded for the different surface covers

The saltation during the aeolian experiment was measured by the number of impact-particles (saltators) in the size range of ~80–500 μm (in accordance with the wind threshold velocity used in this study). The impact-particles include not only loose sand particles but also sand-sized aggregates that participate in saltation. For a better understanding of PM10 emission under soil aggregation, Pearson correlation coefficient between the amount of different aggregate sizes in the topsoil (based on ASD, Fig. 3) and PM10 flux (Table 1) was examined. At the lower wind velocity (32 Hz), none of the aggregate size fractions were correlated with PM10 fluxes. In order to transport aggregates, the wind needs to exceed a certain threshold velocity that depends on the size of the aggregate. The lack of correlation indicates that the wind at 32 Hz was below the threshold velocity even for the smallest aggregates (> 63 μm). Therefore, it is assumed that the PM10 flux in this case is contributed mainly by the direct aerodynamic lifting mechanism. At higher wind velocity (44 Hz), relatively strong correlations were found between PM10 fluxes and the amounts of aggregate at the sizes of <63 μm (R p  = 0.89, p < 0.05) and 250–500 μm (R p  = 0.87, p < 0.05). The correlation between PM10 flux and the size fraction of <63 μm can be explained by the fact that the particles smaller than 10 μm are a part of the fraction of <63 μm. The amplification of wind velocity (from 32 to 44 Hz) enabled the saltation of aggregates up to the size range of 500 μm (Kok et al., 2012; Katra et al., 2014). Aggregates at this size range can enter saltation and release more PM10 particles. Tisdall and Oades (1982) suggested that micro-aggregates (< 250 μm) can be easily eroded as a result of their small size, but on the other hand have higher internal strength than macro-aggregates (>250 μm) as a result of stronger bonds between the particles. The results of the correlation obtained for 250–500 μm aggregate size support this concept, enabling dust emission from aggregates by saltation bombardment and/or self-breakdown and disaggregation.

Conclusions

Dust emission was examined in a study area with typical soil characteristics of arid dust sources. The results highlight variations in PM10 emission due to surface compositions and topsoil disturbance. Surfaces with cover of sparse vegetation (SV) were found to be less resistant to aeolian wind erosion with the highest PM10 fluxes compared to surfaces with cover of rock fragments (RF) cover and mechanical crust (MC). In all surfaces, the disturbance of the natural topsoil caused to decrease in the topsoil aggregation and increased PM10 emission. The amount of loose PM10 particles available at the surface for direct aerodynamic lifting and the amount of the less-stable aggregate size fractions (250–500 μm) are important factors for dust emission rates from these soils. The findings suggest that the specific aggregate size distribution of the soil is necessary for better estimation of PM10 fluxes at the fine scale in arid soils. Calculations of the potential soil loess in this study highlight a direct impact of a short-term topsoil disaggregation on wind erosion. Dust deposition in the Negev, originates from different sources (such as Saharan dust storms) is about 150 g m−2 per year, in which the PM10 fraction is ~25 %. The high dust emission rates from disturbed soils in the Negev suggest a negative balance per year with significant reduction in topsoil PM10 contents (Katra et al., 2016). A major consequence is related to reduction of clays and nutrients that play a key role in the soil stability and fertility in resource-limited ecosystems. The study findings have implications for modeling dust emission from source areas with complex surfaces, which are typical to many dust sources in deserts thorough the world.