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Preparation and magnetic properties of hybrid FeSiBCr amorphous Soft magnetic composites with carbonyl iron and reduced iron particles

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Abstract

Amorphous Soft magnetic composites have the advantages of high resistance, excellent saturation magnetization, and low coercivity. However, due to the high amorphous hardness, the compression density of the soft magnetic composite prepared by it is low. In order to improve the difficulty of pressing amorphous Soft magnetic composites, the Soft magnetic composites with excellent soft magnetic properties and high pressing density were prepared by adding reduced iron powder and carbonyl iron powder to the amorphous powders of FeSiBCr in this work. The results show that the density of Soft magnetic composites with 20 wt% reduced iron powder increases by 14.2%, and the density of Soft magnetic composites with 20 wt% carbonyl iron powder increases by 13.5%. The Soft magnetic composites because of the addition of reduced iron powder with 30 wt% has a higher real permeability of 63 and a lower virtual permeability of 4.77. The Soft magnetic composites with 20 wt% carbonyl iron powder added have the highest real permeability of 55 and the lowest virtual permeability of 0.95. The real part value of the soft magnetic composite without adding iron powder is 23.7% lower than that of the Soft magnetic composites with 20 wt% reduced iron powder, and 18% lower than that of the Soft magnetic composites with 20 wt% carbonyl iron powder. When the carbonyl iron powder content is 20 wt%, the Soft magnetic composites of carbonyl iron powder have the lowest magnetic loss value of 20.6 W/kg and the highest quality factor of 58 (Bm = 0.05T, f = 100 kHz). The magnetic loss of Soft magnetic composites with 20 wt% reduced iron powder (416.3 W/kg) is 39% higher than that of carbonyl iron powder with 20 wt% reduced iron powder (254.2 W/kg) (Bm = 0.05T, f = 200 kHz).

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Data availability

The datasets analyzed during the current study are available from the corresponding author on reasonable request.

References

  1. S. Vovk, S. Dobák, J. Füzer, P. Kollár, R. Bureš, M. Fáberová, Loss separation and thermal studies of Fe/SiO2/ferrite soft magnetic composites. J. Alloys Compd. 945, 169254 (2023)

    Article  CAS  Google Scholar 

  2. H. Shokrollahi, K. Janghorban, Soft magnetic composite materials (SMCs). J. Mater. Process. Technol. 189, 169103 (2007)

    Article  Google Scholar 

  3. J. Yanyan Wang, X. Wang, S. Li, S. Liu, T. Guan, Zhang, Mechanical behavior of Fe80P20/α-Fe amorphous/nanocrystalline composites studied by molecular dynamics simulations. J. Non Cryst. Solids. 606, 122205 (2023)

    Article  Google Scholar 

  4. G. Herzer, Modern soft magnets: amorphous and nanocrystalline materials. Acta Mater. 61, 718–734 (2013)

    Article  CAS  Google Scholar 

  5. H.J. Woo, S.W. Kim, C.P. Kim, D.H. Choi, S. Kim, B.W. Lee, Formation of mixed-powder composites with improved magnetic properties by adding carbonyl iron powders to FeSiCrB amorphous powder. J. Magn. Magn. Mater. 565, 170181 (2023)

    Article  Google Scholar 

  6. Z. Msetra, N. Khitouni, A. Alsawi, M. Khitouni, V. Optasanu, J.-J. Suñol, M. Chemingui, Structural, microstructural, and magnetic properties of nanocrystalline-amorphous Fe–Co–Ta–B alloy processed by high-energy mechanical alloying. J. Mater. 26, 8934–8943 (2023)

    CAS  Google Scholar 

  7. J. Liu, Y. Dong, P. Wang, Z. Zhu, J. Pang, X. Li, J. Zhang, Improved high-frequency magnetic properties of FeSiBCCr amorphous soft magnetic composites by adding carbonyl iron powders. J. Non Cryst. Solids. 605, 122166 (2023)

    Article  CAS  Google Scholar 

  8. Z. Zheng, S. Li, K. Peng, Magnetic properties regulation and loss contribution analysis of FeSi soft magnetic composites doped by carbonyl iron powders. J. Magn. Magn. Mater. 568, 170423 (2023)

    Article  CAS  Google Scholar 

  9. S. Wu, A. Sun, F. Zhai, J. Wang, Q. Zhang, W. Xu, P. Logan, A.A. Volinsky, Annealing effects on magnetic properties of silicone-coated iron-based soft magnetic composites. J. Magn. Magn. Mater. 324, 818–822 (2012)

    Article  CAS  Google Scholar 

  10. S. Wu, X. Sun, Z. Dong, J. Liu, J. Fan, X. Zhou, Y. Wang, A. Sun, Magnetic properties of Fe/parylene soft magnetic composites prepared via chemical vapor deposition. J. Magn. Magn. Mater. 584, 171100 (2023)

    Article  CAS  Google Scholar 

  11. S. Wu, A. Sun, W. Xu, Q. Zhang, F. Zhai, P. Logan, A.A. Volinsky, Iron-based soft magnetic composites with Mn–Zn ferrite nanoparticles coating obtained by sol–gel method. J. Magn. Magn. Mater. 324, 3899–3905 (2012)

    Article  CAS  Google Scholar 

  12. A.H. Taghvaei, H. Shokrollahi, K. Janghorban, H. Abiri, Eddy current and total power loss separation in the iron–phosphate–polyepoxy soft magnetic composites. Mater. Des. 30, 3989–3995 (2009)

    Article  CAS  Google Scholar 

  13. S. Wu, A. Sun, Z. Lu, C. Cheng, X. Gao, Magnetic properties of iron-based soft magnetic composites with SiO2 coating obtained by reverse microemulsion method. J. Magn. Magn. Mater. 381, 451–456 (2015)

    Article  CAS  Google Scholar 

  14. W. Li, S. Xiao, W. Li, Y. Ying, J. Yu, J. Zheng, L. Qiao, J. Li, W. Naoki, J. Wu, S. Che, Hybrid amorphous soft magnetic composites with ultrafine FeSiBCr and submicron FeBP particles for MHz frequency power applications. J. Magn. Magn. Mater. 555, 169365 (2022)

    Article  CAS  Google Scholar 

  15. S. Li, R. Liu, X. Xiong, Preparation and characterization of carbonyl iron soft magnetic composites with magnesioferrite insulating coating layer. J. Mater. 30, 3607–3077 (2020)

    Google Scholar 

  16. S.J. Zhu, F. Duan, J.L. Ni, S.J. Feng, X.S. Liu, Q.R. Lv, X.C. Kan, Soft magnetic composites FeSiAl/MoS2 with high magnetic permeability and low magnetic loss. J. Alloys Compd. 926, 166893 (2022)

    Article  CAS  Google Scholar 

  17. J. Wang, G. Li, Y. He, J. Xu, Z. Qiu, Z. Zheng, M. Xie, Y. Li, Y. Tian, X. Liu, D. Zeng, Improvement in core losses for FeSiAl soft magnetic composites induced by powder annealing treatment. J. Mater. 24, 2500–2513 (2023)

    CAS  Google Scholar 

  18. J. Wang, X. Liu, C. Lei, X. Mao, D. Liu, X. Fan, Z. Luo, F. Luo, Core loss reduction for Fe-6.5wt%Si soft magnetic composites doped with Co element. J. Magn. Magn. Mater. 502, 0304–8853 (2020)

    Article  Google Scholar 

  19. J. Wang, X. Liu, Z. Zheng, Z. Qiu, K. Li, J. Xu, K. Lu, D. Zeng, Reduction of core loss for FeSi soft magnetic composites prepared using atomic layer deposition-based coating and high-temperature annealing. J. Alloys Compd. 909, 164655 (2022)

    Article  CAS  Google Scholar 

  20. L. Li, Z. Gao, A. Li, J. Yi, Y. Ge, Fabrication of carbonyl iron powder/SiO2–reduced iron powder/SiO2 soft magnetic composites with a high resistivity and low core loss. J. Magn. Magn. Mater. 464, 161–167 (2018)

    Article  CAS  Google Scholar 

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Funding

This work was supported by Key Scientific and Technological Project of Henan Province (Grants No: 232102230055), the National Natural Science Foundation of China (Grants No: U1904175), and Key scientific research projects of colleges and universities in Henan Province (24A430050).

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Authors and Affiliations

  1. Henan Key Laboratory of Intelligent Manufacturing of Mechanical Equipment, Institute of Mechanical and Electrical Engineering, Zhengzhou University of Light Industry, Zhengzhou, 450002, China

    Shen Wu, Xiaoran Sun, Jianglei Fan, Xiangkui Zhou, Jianxiu Liu, Yan Wang & Ying Li

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  1. Shen Wu
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  2. Xiaoran Sun
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  3. Jianglei Fan
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  4. Xiangkui Zhou
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  6. Yan Wang
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  7. Ying Li
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Contributions

Shen Wu contributes to conceptualization, methodology, investigation, visualization, and writing-review editing; Xiaoran Sun contributes to conceptualization, methodology, investigation, visualization, and writing-original draft; Jianglei Fan contributes to conceptualization, methodology, investigation, resources, and visualization; Xiangkui Zhou contributes to conceptualization, methodology, investigation, and writing-review editing, supervision; Jianxiu Liu performed formal analysis, date curation, writing-editing, and helped with resources; Yan Wang performed review and contributed to methodology; Ying Li helped with resources.

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Correspondence to Shen Wu.

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Wu, S., Sun, X., Fan, J. et al. Preparation and magnetic properties of hybrid FeSiBCr amorphous Soft magnetic composites with carbonyl iron and reduced iron particles. J Mater Sci: Mater Electron 35, 925 (2024). https://doi.org/10.1007/s10854-024-12666-6

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